Faculty Profiles - AIHARA TAKESHI

写真a

AIHARA TAKESHI

Organization

Institute of Integrated Research Materials and Structures Laboratory Assistant Professor

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Research Interests

Base
Catalyst Chemistry
Solid catalyst
Acid

Research Areas

Nanotechnology/Materials / Inorganic compounds and inorganic materials chemistry
Manufacturing Technology (Mechanical Engineering, Electrical and Electronic Engineering, Chemical Engineering) / Catalyst and resource chemical process

Education

Tokyo Metropolitan University Graduate School of Urban Environmental Sciences Department of Applied Chemistry for Environment

- 2021.3

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Research History

Institute of Science Tokyo Materials and Structures Laboratory, Institute of Integrated Research Assistant Professor

2024.10

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Country：Japan

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Tokyo Institute of Technology Assistant Professor

2023.4 - 2024.9

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Tokyo Institute of Technology Institute of Innovative Research Researcher

2021.4 - 2023.3

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Japan Society for the Promotion of Science

2020.4 - 2021.3

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Papers

Effective Glycerol Carbonate Synthesis From Glycerol and Dimethyl Carbonate Over Rb‐Doped SrTiO3 Nanoparticles Reviewed

Takeshi Aihara, Hideyoshi Kawai, Wataru Aoki, Keigo Kamata

ChemCatChem 18 ( 6 ) e01851 2026.3

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Authorship：Lead author,　Corresponding author Language：English Publishing type：Research paper (scientific journal)

DOI： 10.1002/cctc.202501851

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Significant Enhancement of the Basicity of SrTiO₃ Nanoparticles by Alkali Metal Doping: Implication for the Knoevenagel Condensation Reviewed

Takeshi Aihara, Wataru Aoki, Satoshi Ishikawa, Soungmin Bae, Shin Kiyohara, Yu Kumagai, Michikazu Hara, Keigo Kamata

ACS Applied Nano Materials 8 ( 32 ) 15988 - 15998 2025.8

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Authorship：Lead author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society (ACS)

DOI： 10.1021/acsanm.5c02688

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Ion-Exchanged OMS-1 Nanoparticles for Efficient Aerobic Oxidation Catalysis of Sulfides and Other Organics under Mild Conditions Reviewed

Takumi Nakamura, Keiju Wachi, Takeshi Aihara, Keigo Kamata

ACS Applied Nano Materials 8 ( 17 ) 8728 - 8739 2025.5

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Publishing type：Research paper (scientific journal)

DOI： 10.1021/acsanm.5c00628

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Oxygen Defect Engineering of Hexagonal Perovskite Oxides to Boost Catalytic Performance for Aerobic Oxidation of Sulfides to Sulfones Reviewed

Keiju Wachi, Masashi Makizawa, Takeshi Aihara, Shin Kiyohara, Yu Kumagai, Keigo Kamata

ADVANCED FUNCTIONAL MATERIALS 35 ( 19 ) 2425452 2025.4

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Language：English Publishing type：Research paper (scientific journal)

DOI： 10.1002/adfm.202425452

Web of Science

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La<inf>1-x</inf>Sr<inf>x</inf>FeO<inf>3−δ</inf> Perovskite Oxide Nanoparticles for Low-Temperature Aerobic Oxidation of Isobutane to tert-Butyl Alcohol Reviewed

Masanao Yamamoto, Takeshi Aihara, Keiju Wachi, Michikazu Hara, Keigo Kamata

ACS Applied Materials and Interfaces 16 ( 45 ) 62244 - 62253 2024.11

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Publishing type：Research paper (scientific journal)

DOI： 10.1021/acsami.4c15585

Scopus

PubMed

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Synthesis and catalytic application of nanostructured metal oxides and phosphates Reviewed

Keigo Kamata, Takeshi Aihara, Keiju Wachi

Chemical Communications 60 ( 81 ) 11483 - 11499 2024.9

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Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry (RSC)

This work summarizes catalyst design methodologies based on crystalline complex oxide nanostructures through the synthesis, catalytic application, and structure–activity relationship.

DOI： 10.1039/d4cc03233k

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Copper Phosphate Nanostructures as Catalysts for the Direct Methane Oxidation Reviewed

Aoi Matsuda, Takeshi Aihara, Shin Kiyohara, Yu Kumagai, Michikazu Hara, Keigo Kamata

ACS Applied Nano Materials 7 ( 9 ) 10155 - 10167 2024.5

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Publishing type：Research paper (scientific journal)

DOI： 10.1021/acsanm.4c00549

Scopus

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Acid and base catalysis of SrTiO3 nanoparticles for C–C bond-forming reactions Reviewed

Takeshi Aihara, Wataru Aoki, Michikazu Hara, Keigo Kamata

Catalysis Today 428 114448 - 114448 2024.2

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Authorship：Lead author,　Corresponding author Publishing type：Research paper (scientific journal) Publisher：Elsevier BV

DOI： 10.1016/j.cattod.2023.114448

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Nanosized Ti-Based Perovskite Oxides as Acid–Base Bifunctional Catalysts for Cyanosilylation of Carbonyl Compounds Reviewed

Takeshi Aihara, Wataru Aoki, Shin Kiyohara, Yu Kumagai, Keigo Kamata, Michikazu Hara

ACS Applied Materials & Interfaces 15 ( 14 ) 17957 - 17968 2023.4

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Authorship：Lead author Publishing type：Research paper (scientific journal) Publisher：American Chemical Society (ACS)

DOI： 10.1021/acsami.3c01629

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Continuous Production of Lactic Acid from Glycerol over Bifunctional Catalysts under Base-Free Conditions Using a Liquid-Phase Flow Reactor Reviewed

Erisa Kano, Takeshi Aihara, I. Tyrone Ghampson, Takeyuki Nogami, Hiroki Miura, Tetsuya Shishido

ACS Sustainable Chemistry & Engineering 10 ( 37 ) 12072 - 12081 2022.9

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Publishing type：Research paper (scientific journal) Publisher：American Chemical Society (ACS)

DOI： 10.1021/acssuschemeng.2c00129

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Base-Assisted Aerobic C–H Oxidation of Alkylarenes with a Murdochite-Type Oxide Mg₆MnO₈ Nanoparticle Catalyst Reviewed

Eri Hayashi, Takatoshi Tamura, Takeshi Aihara, Keigo Kamata, Michikazu Hara

ACS Applied Materials & Interfaces 14 ( 5 ) 6528 - 6537 2022.2

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Publishing type：Research paper (scientific journal) Publisher：American Chemical Society (ACS)

DOI： 10.1021/acsami.1c20080

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Lactic Acid Production from Glucose over Y2O3-based Catalysts under Base-free Conditions Reviewed

Daichi HATA, Takeshi AIHARA, Hiroki MIURA, Tetsuya SHISHIDO

Journal of the Japan Petroleum Institute 64 ( 5 ) 280 - 292 2021.9

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Language：English Publishing type：Research paper (scientific journal) Publisher：Japan Petroleum Institute

Methods to catalytic conversion of glucose into lactic acid (LA), which is a versatile platform chemical, have been widely investigated. Herein, various kinds of metal oxide catalysts were used for lactic acid (LA) production from glucose under strong homogeneous base-free conditions. Among the metal oxides tested, Y₂O₃ afforded LA in moderate yield (33 %) together with trioses (dihydroxyacetone and glyceraldehyde) and fructose. It was found that the Y₂O₃/SiO₂ catalyst can effectively catalyze the transformation of glucose into LA. Compared to Y₂O₃, the LA yield was remarkably improved (45 %). The characterization results showed that Y(OH)₃ was highly dispersed on the Y₂O₃/SiO₂ catalyst, acting as a Brønsted base and promoting LA formation from pyruvaldehyde (PA). Brønsted acid sites (hydroxyl groups) located at the interface between Y(OH)₃ and SiO₂ promoted the dehydration of trioses to form PA. The acid and base sites on the Y₂O₃/SiO₂ catalyst functioned in concert to ensure that the overall reaction proceeded efficiently.

DOI： 10.1627/jpi.64.280

CiNii Books

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Brønsted acid property of alumina-based mixed-oxides-supported tungsten oxide Reviewed

Mizuki Saito, Takeshi Aihara, Hiroki Miura, Tetsuya Shishido

Catalysis Today 375 64 - 69 2021.9

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Publishing type：Research paper (scientific journal) Publisher：Elsevier BV

DOI： 10.1016/j.cattod.2020.02.009

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Metal–support cooperation in Al(PO3)3-supported platinum nanoparticles for the selective hydrogenolysis of phenols to arenes Reviewed

Xiongjie Jin, Rio Tsukimura, Takeshi Aihara, Hiroki Miura, Tetsuya Shishido, Kyoko Nozaki

Nature Catalysis 4 ( 4 ) 312 - 321 2021.4

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Publishing type：Research paper (scientific journal) Publisher：Springer Science and Business Media LLC

DOI： 10.1038/s41929-021-00598-x

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Other Link： http://www.nature.com/articles/s41929-021-00598-x
Investigation of the mechanism of the selective hydrogenolysis of C–O bonds over a Pt/WO3/Al2O3 catalyst Reviewed

Takeshi Aihara, Hiroki Miura, Tetsuya Shishido

Catalysis Today 352 73 - 79 2020.8

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Publishing type：Research paper (scientific journal) Publisher：Elsevier BV

DOI： 10.1016/j.cattod.2019.10.008

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Highly active and durable WO₃/Al₂O₃catalysts for gas-phase dehydration of polyols Reviewed

Takeshi Aihara, Katsuya Asazuma, Hiroki Miura, Tetsuya Shishido

RSC Advances 10 ( 61 ) 37538 - 37544 2020

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Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry (RSC)

<p>Gas-phase glycerol dehydration over WO₃/Al₂O₃catalysts was investigated.</p>

DOI： 10.1039/d0ra08340b

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Effect of perimeter interface length between 2D WO₃ monolayer domain and γ-Al₂O₃ on selective hydrogenolysis of glycerol to 1,3-propanediol Reviewed

Takeshi Aihara, Hiroki Miura, Tetsuya Shishido

Catalysis Science & Technology 9 ( 19 ) 5359 - 5367 2019

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Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry (RSC)

<p>The perimeter interface between WO₃ and γ-Al₂O₃ was found to play an important role in selective hydrogenolysis of glycerol to 1,3-propanediol.</p>

DOI： 10.1039/c9cy01385g

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Selective hydrogenolysis of tetrahydrofurfuryl alcohol on Pt/WO 3 /ZrO 2 catalysts: Effect of WO 3 loading amount on activity Reviewed

Shixiang Feng, Aiko Nagao, Takeshi Aihara, Hiroki Miura, Tetsuya Shishido

Catalysis Today 303 207 - 212 2018.4

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Publishing type：Research paper (scientific journal) Publisher：Elsevier BV

DOI： 10.1016/j.cattod.2017.08.058

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Effect of WO₃ Loading on the Activity of Pt/WO₃/Al₂O₃ Catalysts in Selective Hydrogenolysis of Glycerol to 1,3-Propanediol Reviewed

Takeshi Aihara, Hayato Kobayashi, Shixiang Feng, Hiroki Miura, Tetsuya Shishido

Chemistry Letters 46 ( 10 ) 1497 - 1500 2017.10

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Publishing type：Research paper (scientific journal) Publisher：The Chemical Society of Japan

DOI： 10.1246/cl.170601

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MISC

低級アルカンをアルコールへと変換できる安価な鉄触媒の開発 : 高原子価鉄を含むペロブスカイト酸化物ナノ粒子の合成と触媒応用

鎌田慶吾, 和知慶樹, 山本昌尚, 相原健司

クリーンエネルギー / クリーンエネルギー編集委員会編 34 ( 4 ) 34 - 39 2025.4

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Language：Japanese Publisher：東京 : 日本工業出版

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Other Link： https://ndlsearch.ndl.go.jp/books/R000000004-I034044098
Selective Oxidation of Methane into Formaldehyde over Copper Phosphate Catalysts

松田蒼依, 相原健司, 原亨和, 鎌田慶吾

日本化学会春季年会講演予稿集(Web) 104th 2024

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J-GLOBAL

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Aerobic oxidation of sulfides catalyzed by Ru-doped hexagonal perovskite oxides

牧澤昌史, 和知慶樹, 相原健司, 鎌田慶吾

日本化学会春季年会講演予稿集(Web) 104th 2024

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J-GLOBAL

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Effect of A-site doping on the acid-base properties of SrTiO₃ nanoparticles

相原健司, 青木航流, 鎌田慶吾

日本化学会春季年会講演予稿集(Web) 104th 2024

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受賞講演不均一系触媒による単糖類からの乳酸一段合成 : 2022年度論文賞—特集 2022年度受賞講演(2)

宍戸哲也, 畑大地, 相原健司, 三浦大樹

ペトロテック = Petrotech : 石油学会情報誌 / 石油学会編 46 ( 10 ) 631 - 636 2023.10

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Language：Japanese Publisher：東京 : 石油学会 ; 1978-

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Other Link： https://ndlsearch.ndl.go.jp/books/R000000004-I033112565
高比表面積Tiペロブスカイトナノ粒子触媒の合成とKnoevenagel縮合反応への応用

青木航流, 相原健司, 鎌田慶吾, 原亨和

触媒討論会予稿集(CD-ROM) 131st 2023

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Ti含有ペロブスカイト酸化物の酸・塩基性質の解明とシアノシリル化反応

相原健司, 青木航流, 鎌田慶吾, 原亨和

触媒討論会予稿集(CD-ROM) 131st 2023

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Synthesis of Ti-based perovskite nanoparticles with high specific surface areas by sol-gel method and their catalytic application to Knoevenagel condensation reaction

青木航流, 相原健司, 鎌田慶吾, 原亨和

日本化学会春季年会講演予稿集(Web) 103rd 2023

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Acid-Base Bifunctionality of Ti-based Perovskite Nanoparticles for Cyanosilylation

相原健司, 青木航流, 鎌田慶吾, 原亨和

日本化学会春季年会講演予稿集(Web) 103rd 2023

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SrTiO₃ナノ粒子の酸塩基性質とKnoevenagel縮合反応への応用

青木航流, 相原健司, 原亨和, 鎌田慶吾

触媒討論会予稿集(CD-ROM) 132nd 2023

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高原子価鉄を含むペロブスカイト酸化物触媒を用いた低級アルカンの液相酸化反応

山本昌尚, 相原健司, 原亨和, 鎌田慶吾

触媒討論会予稿集(CD-ROM) 132nd 2023

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リン酸銅触媒を用いたメタンからホルムアルデヒドの直接合成と反応機構解明

松田蒼依, 相原健司, 原亨和, 鎌田慶吾

触媒討論会予稿集(CD-ROM) 132nd 2023

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Synthesis of Murdochite-type Oxide Mg₆MnO₈ Nanoparticles and the Catalytic Oxidation Properties

林愛理, 相原健司, 田村高敏, 鎌田慶吾, 原亨和

日本化学会春季年会講演予稿集(Web) 102nd 2022

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ペロブスカイト酸化物の酸塩基性質によるシアノシリル化反応

相原健司, 青木航流, 鎌田慶吾, 原亨和

触媒討論会討論会A予稿集(CD-ROM) 130th 2022

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J-GLOBAL

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Crystalline Metal Oxide Catalysts for Organic Synthesis

Keigo Kamata, Takeshi Aihara

Crystalline Metal Oxide Catalysts 219 - 271 2022

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Publisher：Springer Nature Singapore

DOI： 10.1007/978-981-19-5013-1_8

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Other Link： https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-21H01713/
Study on the reaction mechanism of hydrogenolysis on Pt/WO₃/Al₂O₃ catalysts

Aihara Takeshi, Miura Hiroki, Shishido Tetsuya

Proceeding of Annual/Fall Meetings of the Japan Petroleum Institute 2018f 95 2018

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Language：Japanese Publisher：The Japan Petroleum Institute

In this study, to reveal the reaction mechanism of hydrogenolysis over Pt/WO₃/Al₂O₃ catalyst, the effect of substrate structure on the activity was investigated. The activity differences of substrates with different positions of OH groups and number of carbon were compared. The reaction pathway of glycerol hydrogenolysis was also estimated from kinetics study. From these investigation, the reaction mechanism in hydrogenolysis of biomass compounds was estimated.

DOI： 10.11523/sekiyu.2018f.0_95

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Awards

第13回 GSC Student Travel Grant Award

2020 Japan Association for Chemical Innovation (JACI)

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第8回 CSJ化学フェスタ2017 優秀ポスター賞

2019.10 The Chemical Society of Japan

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Poster Award 1st Prize

2018.7 ISHHC18 Role of perimeter interfaces between WO3 monolayer domain and Al2O3 in hydrogenolysis of glycerol by Pt/WO3/Al2O3 catalysts

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第7回 CSJ化学フェスタ2017 優秀ポスター賞

2017.10 公益社団法人日本化学会

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学生ポスター発表賞

2017.3

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Research Projects

Creation of innovative reaction field based on nano-structure control of multicomponent metal oxide catalysts

Grant number：24H00393 2024.4 - 2028.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for Scientific Research (A)

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Grant amount：\48230000 （ Direct Cost: \37100000 、 Indirect Cost：\11130000 ）

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ドーピングによるペロブスカイト酸化物の活性点制御と高機能酸塩基触媒の開発

Grant number：24K17557 2024.4 - 2026.3

日本学術振興会科学研究費助成事業若手研究

相原健司

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Grant amount：\4680000 （ Direct Cost: \3600000 、 Indirect Cost：\1080000 ）

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環境調和型触媒への応用を指向したペロブスカイト酸化物の開発

2023.9 - 2024.3

東京工業大学基礎研究機構広域基礎研究塾新研究挑戦奨励金

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ペロブスカイト酸化物の表面イオン種の制御と有機化学反応への利用

2023.8 - 2025.3

一般財団法人イオン工学振興財団 2023年度研究助成

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Authorship：Principal investigator

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ペロブスカイト型複合酸化物の歪みを利用した酸・塩基性質の精密制御

Grant number：21K20482 2021.8 - 2023.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for Research Activity Start-up Grant-in-Aid for Research Activity Start-up

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Grant amount：\2990000 （ Direct Cost: \2300000 、 Indirect Cost：\690000 ）

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反応場を精密制御した機能性触媒によるバイオマス資源の選択的水素化分解

Grant number：20J13086 2020.4 - 2022.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for JSPS Fellows Grant-in-Aid for JSPS Fellows

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Grant amount：\2300000 （ Direct Cost: \2300000 ）

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