Faculty Profiles - MICHINOBU TSUYOSHI

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MICHINOBU TSUYOSHI

Organization

School of Materials and Chemical Technology Professor

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News & Topics

大気下での安定性に優れた電子輸送型高分子トランジスタの開発に成功有機エレクトロニクス研究における標準物質としての利用を期待

2019/08/08

Languages： Japanese

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アクセプター性骨格のみからなる高分子構造を設計環境負荷が低い直接アリール化重縮合による効率的な合成に成功異性体構造によるトランジスタ性能の違いを実証室温大気下で1ヵ月保存後でも十分な電子移動度を保持する安定な高分子トランジスタの開発に成功
New synthesis method opens up possibilities for organic electronics

2019/08/07

Languages： English

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Scientists at Tokyo Institute of Technology (Tokyo Tech) modify a previous synthesis method to create a new semiconducting polymer with remarkable properties which could be used in organic electronic devices such as thin film transistors.
Organic electronics: Scientists develop a high-performance unipolar n-type thin-film transistor

2019/03/01

Languages： English

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Researchers at Tokyo Tech report a unipolar n-type transistor with a world-leading electron mobility performance of up to 7.16 cm2 V?1 s?1. This achievement heralds an exciting future for organic electronics, including the development of innovative flexible displays and wearable technologies.
水素結合を利用して高分子トランジスタを開発デジタル回路や熱電変換素子、太陽電池などへの応用にめど

2019/02/27

Languages： Japanese

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電子移動度7.16 cm2 V-1 s-1の電子輸送型高分子トランジスタを開発分子内水素結合を利用することで高分子の平面性を最適化非常に小さい分子間距離3.40Aを有する結晶性薄膜を形成
New semiconducting polymers with record-setting electron mobility for future devices

2018/02/22

Languages： English

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Scientists at Tokyo Tech have successfully developed n-type semiconducting copolymers with high electron mobilities. They investigated their properties and their effectiveness for thin-film transistors, obtaining highly promising results.
高い電子移動度を持つ有機半導体高分子を開発全有機高分子型のデジタル回路や太陽電池などへの応用に期待

2018/02/16

Languages： Japanese

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窒素原子の配置を工夫してエネルギー準位や分子の平面性を最適化アミノアルキル単分子膜で電子のみ輸送可能にこの有機半導体高分子[用語1]で高性能な有機トランジスタの開発に成功

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Degree

Doctor of Engineering ( 2003.3 Waseda University )

Research Interests

Organic materials, Polymer chemistry

Research Areas

Manufacturing Technology (Mechanical Engineering, Electrical and Electronic Engineering, Chemical Engineering) / Electron device and electronic equipment
Nanotechnology/Materials / Polymer materials
Nanotechnology/Materials / Functional solid state chemistry
Nanotechnology/Materials / Polymer chemistry

Education

Waseda University Graduate School of Science and Engineering

2000.4 - 2003.3

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Waseda University Graduate School of Science and Engineering

1999.4 - 2000.3

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Waseda University School of Science and Engineering

1995.4 - 1999.3

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Research History

Institute of Science Tokyo Professor

2024.10

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Tokyo Institute of Technology Professor

2023 - 2024.9

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Country：Japan

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Tokyo Institute of Technology Associate Professor

2012 - 2023

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Tokyo Institute of Technology

2008 - 2012

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Tokyo University of Agriculture and Technology

2006 - 2008

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物質・材料研究機構博士研究員

2005 - 2006

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スイス連邦工科大学チューリッヒ校博士研究員

2003 - 2005

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Professional Memberships

THE SOCIETY OF FIBER SCIENCE AND TECHNOLOGY, JAPAN

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高分子学会

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日本化学会

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Papers

Simultaneous Enhancement of Electron and Hole Mobility in Para ‐Azaquinodimethane‐Derived Polymer by Individually Applying Various Additives

Qian Liu, Waner He, Shuangzhe Zhang, Yongheng Zhou, Lei Li, Xiaolong Chen, Katsuki Yaginuma, Yi Lu, Hideyuki Otsuka, Hidetoshi Matsumoto, Dou Luo, Prashant Sonar, Tsuyoshi Michinobu, Aung Ko Ko Kyaw

Advanced Materials 2026.1

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Publishing type：Research paper (scientific journal) Publisher：Wiley

ABSTRACT

Achieving simultaneous enhancement of electron and hole mobility in organic semiconductors (OSCs) using a single additive remains a significant challenge. In this study, we present a unique additive strategy that enables concurrent improvement of both n‐ and p‐type transport in an n‐dominant ambipolar polymer incorporating para ‐azaquinodimethane and diketopyrrolopyrrole. By individually applying various additives including ionic, p‐type, and n‐type compounds, we achieve unprecedented enhancements of both electron (∼400%) and hole (∼100%) mobility. Such parallel improvement is unattainable via conventional electron transfer mechanism. We ascribe this effect to optimized film morphology, reduced activation energy, and lowered contact resistance. To further elucidate additive‐induced variations in electronic structure and guide future molecular design, density functional theory calculations reveal that incorporating para ‐azaquinodimethane into the polymer backbone facilitates strong orbital coupling with additives. This coupling introduces additional charge transport pathways between polymer segments, enhancing both electron and hole transport along lamellar and π–π stacking directions. Our findings suggest promoting robust orbital coupling between host polymers and additives offers a promising strategy to concurrently boost electron and hole mobility in a single OSC, effectively circumventing traditional limitations associated with separate p‐ and n‐type additives/dopants.

DOI： 10.1002/adma.202513065

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Sustainable Nonenantioselective Production and Stereochemical Characterization of the Lignin‐Derived Chiral Building Block 3‐Carboxymuconolactone

Yuzo Suzuki, Takuma Araki, Masaya Fujita, Naofumi Kamimura, Eiji Masai, Tsuyoshi Michinobu, Yuichiro Otsuka, Shojiro Hishiyama, Masaya Nakamura

ChemistryOpen 15 ( 1 ) 2026.1

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Publishing type：Research paper (scientific journal) Publisher：Wiley

To promote the comprehensive utilization of renewable lignocellulosicbiomass, a practical technology for the nonenantioselective production of 3‐carboxymuconolactone (3CML), a lignin‐derived chiral building block, is presented. Although an engineered Pseudomonas putida strain with plasmids containing bacterial and fungal genes was previously used to convert lignin‐derived aromatic compounds into optically pure 4 S ‐3CML, using the enantiomeric pair 4 S ‐3CML and 4 R ‐3CML as polymer building blocks in appropriate blending ratios can be expected to afford novel materials such as polylactic acid with tunable physical properties for targeted applications. Therefore, in this study, P. putida was engineered to convert vanillic acid, the major aromatic compound derived from lignin, into 3‐carboxy‐ cis , cis ‐muconate, which was then chemically converted into racemic 3CML under acidic conditions. Using a chiral high performance liquid chromatography–circulardichroism system, racemic 3CML was stereochemically characterized on the basis of the enantiomers. A one‐pot process for the production of racemic 3CML was established by combining fed‐batch fermentation with subsequent acidic treatment using a jar fermenter, affording 6.6 g/L 4 S ‐3CML and 7.2 g/L 4 R ‐3CML in a high yield of 93.1%. The developed process can be consistently performed at 28°C without requiring pressure or metal reagents and allows using a reduced volume of solvent, offering clear advantages for industrial applications.

DOI： 10.1002/open.202500453

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Effects of alkylene spacer length of 2-pyrone-4,6-dicarboxylic acid polyesters on biodegradability and metal adhesive properties Invited Reviewed

Yijie Jin, Keiju Yoshida, Suzuha Kimura, Atsushi Isobe, Keiichi Kuboyama, Masaya Fujita, Takuma Araki, Yuzo Suzuki, Yuichiro Otsuka, Naofumi Kamimura, Eiji Masai, Masaya Nakamura, Tsuyoshi Michinobu

NPG Asia Materials 17 ( 1 ) 2025.12

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Springer Science and Business Media LLC

Abstract

2-Pyrone-4,6-dicarboxylic acid (PDC) is a lignin-derived biometabolic intermediate that can be produced on a large scale by using transforming bacteria and can be directly polymerized by polycondensation with diols to produce biomass polyesters. In the present study, a variety of PDC-based polyesters were successfully synthesized by direct polymerization between PDC and diols with different alkyl chain lengths. The thermal, crystalline, and mechanical properties of a series of PDC polyesters were fully characterized. The biodegradability of the PDC polyesters was investigated by biodegradation tests in a confined simulated environment using pond water. There was a clear correlation between the biodegradation rate, alkylene spacer length, and polymer hydrophilicity. In addition, the PDC polyesters exhibited excellent adhesive properties to various metals, and their adhesive properties gradually decreased with a decrease in the PDC content in the polymers. The excellent adhesion to an aluminum plate with the lap-shear strength of up to 15.26 MPa was demonstrated and this value is comparable to those of the-state-of-the-art commercial quick-drying metal adhesives.

DOI： 10.1038/s41427-025-00626-3

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Other Link： https://www.nature.com/articles/s41427-025-00626-3
Donor–Acceptor–Donor Small-Molecular Dots are Brighter than Polymer Dots of Similar Chromophore Units Reviewed

Nirmal K. Das, Hubert Piwoński, Shuho Nozue, Manjusha Joshi, Kosuke Terayama, Tsuyoshi Michinobu, Satoshi Habuchi

ACS Applied Materials & Interfaces 17 ( 49 ) 67010 - 67026 2025.11

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Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society (ACS)

DOI： 10.1021/acsami.5c17687

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Synthesis of pyridine-based push-pull chromophores via [2 + 2] cycloaddition-retroelectrocyclization and their p-doping performance in poly(3-hexylthiophene-2,5-diyl) Reviewed International journal

Xu Chen, Takashi Iwahashi, Momoka Isobe, Kaname Kanai, Tsuyoshi Michinobu

Dyes and Pigments 242 112973 2025.11

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Elsevier

DOI： 10.1016/j.dyepig.2025.112973

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Thermal degradation mechanism and isothermal sublimation kinetics of DDMEBT: Structure–property correlations for process optimization Reviewed

Laura Nistor, Cătălin Lisa, Tsuyoshi Michinobu, Gabriela Lisa

Journal of Materials Research and Technology 39 7261 - 7276 2025.11

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Language：English Publishing type：Research paper (scientific journal) Publisher：Elsevier BV

DOI： 10.1016/j.jmrt.2025.11.046

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All‐Solution Processed OFETs from Non‐Chlorinated Solvents Based on New Isoindigo‐Based Conjugated Polymer Reviewed

Katherina Haase, Jonathan Perez Andrade, Mike Hambsch, Vithyasaahar Sethumadhavan, Waner He, Tsuyoshi Michinobu, Prashant Sonar, Stefan C. B. Mannsfeld

Advanced Electronic Materials 11 ( 18 ) 2025.9

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Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

Abstract

Here, an Isoindigo (IID) comprised with Naphthodithiophene (NDT)‐based low band‐gap donor–acceptor copolymer semiconductor is designed, synthesized, and investigated. The newly reported polymer provides good solubility in a range of halogenated and non‐halogenated solvents due to the attachment of long branched alkyl chains on the Isoindigo core. After optimizing the performance of organic field effect transistors (OFETs) through the use of high‐boiling‐point chlorinated solvents, A similar approach is followed to realize transistors without the need of using halogenated solvents as a green approach. Well‐working transistors are shown with mobility values in a similar range as obtained for OFETs with films prepared from halogenated solvents, while significantly reducing the environmental impact. Finally, all‐solution‐processed, flexible OFETs are prepared without the use of halogenated solvents, which is an important step in the view of potential large area production of flexible electronics.

DOI： 10.1002/aelm.202500375

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Enhanced Photoresponsive Transistor Memory Performance through [2 + 2] Cycloaddition–Retroelectrocyclization of Tröger’s Base-Carbazole Copolymer Reviewed International coauthorship International journal

Chia-Yang Lin, Mei-Nung Chen, Joost Kimpel, Waner He, Guey-Sheng Liou, Yu-Cheng Chiu, Tsuyoshi Michinobu

ACS Applied Polymer Materials 7 ( 14 ) 9286 - 9293 2025.7

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acsapm.5c01667

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Synthesis of Water-Soluble Cyano-Containing Polymeric Additives and Their Application to the Preparation of Ag+-Loaded Hydrogels Reviewed International journal

Xu Chen, Yuuki Hata, Hidetoshi Matsumoto, Takeshi Serizawa, Tsuyoshi Michinobu

ACS Applied Polymer Materials 7 ( 12 ) 8245 - 8253 2025.6

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acsapm.5c01383

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Vinylene-bridged naphthalenediimide-based dual-acceptor copolymers for thin-film transistors and solar steam generation Invited Reviewed

Chia-Yang Lin, Guan-Lin Wu, Ting-Yu Wang, Waner He, Ying-Sheng Wu, Shunsuke Imaoka, Shohei Shimizu, Wen-Chang Chen, Yoshimitsu Sagara, Chu-Chen Chueh, Tsuyoshi Michinobu

RSC Applied Polymers 3 ( 4 ) 1011 - 1018 2025.6

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry (RSC)

In a series of studies on vinylene-bridged dual-acceptor copolymers, high transistor mobilities were observed in highly crystalline polymers, and high solar-to-vapor conversion efficiencies were achieved in narrow bandgap polymers.

DOI： 10.1039/d5lp00136f

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Rhodium‐Catalyzed Intermolecular Arylative [2 + 2 + 1] Annulation–Oxidation to Produce Electron‐Deficient Azulene‐Embedded Polycyclic Aromatic Hydrocarbons Reviewed

Yoshinobu Kamiya, Yu Sato, Tomohiro Oriki, Yuko Kishida, Haruki Sugiyama, Waner He, Kexiang Zhao, Tsuyoshi Michinobu, Hidehiro Uekusa, Ken Tanaka

Angewandte Chemie International Edition 64 ( 29 ) 2025.5

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Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

Abstract

Azulene derivatives have attracted much attention for their application in organic electronic materials and devices because of their large dipole moment and small HOMO–LUMO energy gap. As these physical properties of azulene depend on its substitution and condensation patterns, developing methods to synthesize functionalized and π‐extended azulenes is desirable. However, synthesizing π‐extended azulenes requires harsh reaction conditions, making it hard to achieve both functionalization and π‐extension. Here, we report the synthesis of electron‐deficient azulene‐embedded polycyclic aromatic hydrocarbons (PAHs) with two alkoxycarbonyl groups by the rhodium‐catalyzed intermolecular arylative [2 + 2 + 1] annulation of teraryl diynes with dialkyl acetylenedicarboxylates followed by oxidation at room temperature. Interestingly, for the electron‐rich diyne, prolonged oxidation time after the arylative [2 + 2 + 1] annulation yields a helicene‐like bis(azulene‐embedded PAH) in good yield. Thus, obtained electron‐deficient fused azulenes have small HOMO–LUMO energy gaps (up to E _g ^elec = 1.52 and E _g ^theo = 2.06), resulting in long‐wavelength absorption extending into the near‐infrared region. Due to bulky electron‐withdrawing groups and π‐extension, the molecule becomes saddle‐shaped and highly polarized, and strong π–π stacking interactions are observed in both the solid and solution states.

DOI： 10.1002/anie.202505622

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Accelerated Development of Novel Biomass-Based Polyurethane Adhesives via Machine Learning Reviewed International journal

Ye Cheng, Takuma Araki, Naofumi Kamimura, Eiji Masai, Masaya Nakamura, Sergei Manzhos, Tsuyoshi Michinobu

ACS Applied Materials & Interfaces 17 ( 10 ) 15959 - 15968 2025.3

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acsami.4c20371

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Synthesis of Nonplanar Push–Pull Chromophores with Various Heterocyclic Moieties via [2 + 2] Cycloaddition-Retroelectrocyclization Reaction Reviewed International journal

Xu Chen, Tsuyoshi Michinobu

The Journal of Organic Chemistry 90 ( 4 ) 1561 - 1570 2025.1

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acs.joc.4c02595

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Improved thermal properties of polydimethylsiloxane by copolymerization and thiol–ene crosslinking of 2-pyrone-4,6-dicarboxylic acid moiety Invited Reviewed International journal

Takahiro Shimura, Yijie Jin, Keiichi Kubyama, Takuma Araki, Naofumi Kamimura, Eiji Masai, Masaya Nakamura, Tsuyoshi Michinobu

Polymer Chemistry 16 45 - 51 2025

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry

DOI： 10.1039/D4PY01051E

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Enhanced Photothermal Property of Dithienoindacenodithiophene Molecules by [2 + 2] Cycloaddition–Retroelectrocyclization Reaction for Efficient Solar Steam Generation Invited Reviewed International journal

Chia Yang Lin, Shohei Shimizu, Yoshimitsu Sagara, Hidetoshi Matsumoto, Tsuyoshi Michinobu

Solar RRL 9 ( 5 ) 2400803 2025

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

DOI： 10.1002/solr.202400803

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Synthesis, Characterization, and Thin‐Film Properties of Post‐Functionalized N,N‐Dimethylanilinoethynyl‐Substituted Cyclobutenofullerenes Invited Reviewed International journal

Michio Yamada, Haruki Sakuma, Waner He, Hiromichi Araki, Yutaka Maeda, Mitsuaki Suzuki, Tsuyoshi Michinobu

Chemistry – An Asian Journal 20 ( 3 ) e202401111 2024.11

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Authorship：Last author Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

Abstract

A π‐extended cyclobutenofullerene containing an N,N‐dimethylanilinoethynyl group was synthesized via a one‐pot cascade reaction of C₆₀ with the corresponding propargylic phosphate. The cyclobutenofullerene was further modified using either one‐pot or sequential post‐functionalization methods, yielding derivatives containing altered addend structures. During one‐pot post‐functionalization, hydration reaction of the alkyne moiety continued after the formation of cyclobutenofullerenes. The sequential post‐functionalization approach involved introducing the tetracyanobutadiene structure through formal [2+2] cycloaddition and a subsequent retroelectrocyclization reaction with tetracyanoethylene. The electronic and optical properties of the derivatives in solution, as well as their field‐effect transistor behavior in thin films, were thoroughly assessed to elucidate the optoelectronic differences arising from various addend structures. The properties of the three characteristic cyclobutenofullerene derivatives in the solution and thin films significantly varied depending on the addends. Among the three derivatives studied, only cyclobutenofullerene, featuring a folded structure induced by the hydration of the alkyne moiety, exhibited n‐type semiconductor behavior in the thin films. The findings of this study present a novel methodology for synthesizing and functionalizing fullerene derivatives, together with a conceptual framework for tailoring molecular properties.

DOI： 10.1002/asia.202401111

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A facile membraneless method for detecting alkali-metal cations using organic electrochemical transistors Invited Reviewed International coauthorship International journal

Waner He, Yurika Kashino, Naoya Nozaki, Joost Kimpel, Hidetoshi Matsumoto, Yuhei Hayamizu, Tsuyoshi Michinobu

Journal of Materials Chemistry C 12 18282 - 18290 2024.10

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry

DOI： 10.1039/D4TC03047H

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Metal-free double azide addition to strained alkynes of an octadehydrodibenzo[12]annulene derivative with electron-withdrawing substituents Invited Reviewed International journal

Naoki Takeda, Shuichi Akasaka, Susumu Kawauchi, Tsuyoshi Michinobu

Beilstein Journal of Organic Chemistry 20 2234 - 2241 2024.9

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Beilstein-Institut

DOI： 10.3762/bjoc.20.191

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Influence of Vinyl Bridging on Transistor Properties of Naphthalenediimide-Based Dual-Acceptor Copolymers Reviewed International coauthorship International journal

Ying-Sheng Wu, Chu-Yen Tsai, Dao Duy Thanh, Yen-Han Shih, Hsu-Tzu Cheng, Tsuyoshi Michinobu, Wen-Chang Chen, Chu-Chen Chueh

ACS Applied Polymer Materials 6 ( 10 ) 5900 - 5909 2024.5

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Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acsapm.4c00539

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Diketopyrrolopyrrole‐Dioxo‐Benzodithiophene‐Based Multi‐Functional Conjugated Polymers for Organic Field Effect Transistors and Perovskite Solar Cells Invited Reviewed International journal

Kakaraparthi Kranthiraja, Waner He, Hao-Wei Yu, Zhen Feng, Naoya Nozaki, Hidetoshi Matsumoto, Ming-Hsuan Yu, Yong Li, Sergei Manzhos, Mats R. Andersson, Chu-Chen Chueh, Tsuyoshi Michinobu, Prashant Sonar

Solar RRL 8 ( 14 ) 2400185 2024.5

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Authorship：Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

While dual‐acceptor‐type conjugated polymers have witnessed a great success in organic field‐effect transistors (OFETs), their potential multifunctionality in other optoelectronic devices has been overlooked. Herein, we designed, synthesized, and characterised three conjugated polymers (DPPF‐BDD, DPPT‐BDD and DPPSe‐BDD) comprising furan/thiophene/selenophene flanked diketopyrrolopyrrole (DPP) and dioxo‐benzodithiophene (BDD) as repeating units. Modulating the chalcogen on DPP flank showed an impact on dual‐acceptor polymers optoelectronic properties. Subsequently, we investigated the potential of these polymers in both OFETs and perovskite solar cells (PSCs) either as semiconductors or as passivation materials, respectively. Interestingly, DPPF‐BDD, DPPT‐BDD, and DPPSe‐BDD showed ambipolar behaviour in vacuum with hole (μ_h) and electron (μ_e) mobilities of 0.026/0.022, 0.022/0.012 and 0.007/0.005 cm² V^‐1s^‐1, respectively. Upon doping tetrabutylammonium iodide into DPPF‐BDD, DPPT‐BDD and DPPSe‐BDD polymers, the respective OFETs showed relatively higher μ_h and μ_e (0.038/0.050; 0.028/0.025; 0.005/0.015 cm²V^‐1s^‐1) than the undoped polymer OFETs. Furthermore, DPPF‐BDD‐, DPPT‐BDD‐, and DPPSe‐BDD‐incorporated (in the antisolvent treatment and PCBM ETL) PSCs displayed maximum PCE of 23.48%, 22.85% and 23.35%, respectively, surpassing the control device (22.83%), which was benefited from the perovskite surface passivation and the charge extraction improvement. Overall, we present a new class of multifunctional DPP‐based dual‐acceptor‐type polymers that are highly compatible with OFETs and high‐performance PSCs.

This article is protected by copyright. All rights reserved.

DOI： 10.1002/solr.202400185

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Biodegradable and wood adhesive polyesters based on lignin-derived 2-pyrone-4,6-dicarboxylic acid Reviewed International journal

Yijie Jin, Takuma Araki, Naofumi Kamimura, Eiji Masai, Masaya Nakamura, Tsuyoshi Michinobu

RSC Sustainability 2 1985 - 1993 2024.5

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Royal Society of Chemistry

DOI： 10.1039/D4SU00163J

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Self-healing and shape-memory polymers based on cellulose acetate matrix Invited Reviewed

Han Jia, Keiya Jimbo, Hirogi Yokochi, Hideyuki Otsuka, Tsuyoshi Michinobu

Science and Technology of Advanced Materials 25 ( 1 ) 2024.3

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Informa UK Limited

DOI： 10.1080/14686996.2024.2320082

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Revealing the Effect of Halogenation Strategy on the Regulation of Crystallization Kinetics and Molecular Packing for High‐Performance Organic Solar Cells Reviewed International coauthorship International journal

Dou Luo, Lifu Zhang, Jie Zeng, Weijie Chi, Jialing Zhou, Erjun Zhou, Lanqing Li, Takashi Iwahashi, Tsuyoshi Michinobu, Yukio Ouchi, Baomin Xu, Aung Ko Ko Kyaw

Advanced Functional Materials 34 ( 12 ) 2311736-1 - 2311736-16 2024.3

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Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

<jats:title>Abstract</jats:title><jats:p>Halogenation of non‐fused ring electron acceptors (NFREAs) plays an important role in regulating their optoelectronic properties. However, the underlying mechanisms and their impact on the performance of organic solar cells (OSCs) have remained unclear. Herein, a series of halogenated NFREAs incorporating F, Cl, and Br, are prepared to study their effect on crystallization kinetics, phase separation, molecular packing, and charge transport. Among various halogenation strategies, chlorination minimizes the Coulomb attractive energy between donor and acceptor, thereby facilitating exciton dissociation. In situ UV–vis absorption tests reveal that chlorinated acceptors exhibit a longer crystallization time, effectively suppressing excessive molecular aggregation and enhancing overall crystallinity. Additionally, chlorinated acceptors exhibit a longer exciton diffusion length, which promotes exciton dissociation while mitigating charge recombination in the devices. Consequently, two chlorinated NFREAs, TCN‐Cl, and PCN‐Cl, yield an impressive power conversion efficiency (PCE) of 14.85% and 15.30%, respectively, when blended with PM6 and J52 donors. These values represent the highest reported PCEs to date for NFREAs with A‐π‐A’‐π‐A and A‐π‐D‐π‐A structures. The study elucidates the crucial role of chlorination in extending exciton diffusion length and crystallization time. These effects significantly benefit phase separation within the active layers, enhance charge separation, and suppress recombination for achieving high‐efficiency OSCs.</jats:p>

DOI： 10.1002/adfm.202311736

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Enhanced Photothermal Property of NDI-Based Conjugated Polymers by Copolymerization with a Thiadiazolobenzotriazole Unit Invited Reviewed International journal

Mingqian Wang, Chia-Yang Lin, Yoshimitsu Sagara, Tsuyoshi Michinobu

ACS Materials Au 4 ( 1 ) 82 - 91 2024.1

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acsmaterialsau.3c00077

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Ionic Conductive Organogels Based on Cellulose and Lignin-Derived Metabolic Intermediates Reviewed International journal

Han Jia, Keiya Jimbo, Koichi Mayumi, Tatsuro Oda, Toshiki Sawada, Takeshi Serizawa, Takuma Araki, Naofumi Kamimura, Eiji Masai, Eiji Togawa, Masaya Nakamura, Tsuyoshi Michinobu

ACS Sustainable Chemistry and Engineering 12 ( 1 ) 501 - 511 2024.1

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：American Chemical Society

DOI： 10.1021/acssuschemeng.3c06488

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Antioxidative activity of alcohol-soluble fullerene derivative Reviewed

Yoko Yoshitake, Tsuyoshi Michinobu

Fullerenes, Nanotubes and Carbon Nanostructures 32 ( 5 ) 505 - 508 2023.12

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Authorship：Last author,　Corresponding author Language：English Publishing type：Research paper (scientific journal) Publisher：Informa UK Limited

DOI： 10.1080/1536383x.2023.2296945

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Thermal stability and degradation mechanism of <scp>C₆₀</scp> fullerene‐based polymers Reviewed

Gabriela Lisa, Cerasela‐Ionela Cleminte, Tsuyoshi Michinobu

Journal of Applied Polymer Science 141 ( 11 ) 2023.12

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Authorship：Last author Language：English Publishing type：Research paper (scientific journal) Publisher：Wiley

Abstract

In this paper, the thermal stability and degradation mechanisms of C₆₀ fullerene‐based polymers, obtained by click polymerization between dialkyne‐substituted C₆₀ derivative monomers and 1,3,5‐tris(dodecyloxy)benzene‐based diazide comonomers, were evaluated. The activation energy of the fullerene polymer C₆₀P2 with an ethylene spacer, determined under peak degradation rate conditions, was lower than that of the counter polymer C₆₀P1 with a methylene spacer, suggesting lower thermal stability of C₆₀P2. The combined technique of thermogravimetric analysis—mass spectroscopy and Fourier transform infrared spectroscopy revealed that the thermal decomposition onset of the analyzed samples is accompanied by CC cleavage of the dodecyloxyside chain groups, followed by the decomposition of the 1,2,3‐triazole, dicarboxylate and benzoate moieties. It was found that no thermal decomposition of the fullerene carbon cage occurs up to 670°C. Molecular modeling with Hyperchem software version 7.5 confirmed that C₆₀P1 is more thermally stable than C₆₀P2.

DOI： 10.1002/app.55079

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PEDOT:PSS versus Polyaniline: A Comparative Study of Conducting Polymers for Organic Electrochemical Transistors Reviewed International journal

Ryotaro Kawamura, Tsuyoshi Michinobu

Polymers 15 ( 24 ) 4657 2023.12

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DOI： 10.3390/polym15244657

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Structural design of conjugated polymers for fluorescence bioimaging in the second near‐infrared window Invited Reviewed International coauthorship International journal

Kosuke Terayama, Satoshi Habuchi, Tsuyoshi Michinobu

Journal of Polymer Science 61 ( 19 ) 2276 - 2291 2023.10

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DOI： 10.1002/pol.20230421

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Charge transport and near-infrared emission properties of semiconducting polymers Invited Reviewed International journal

Tsuyoshi Michinobu

Polymer Journal 55 1049 - 1056 2023.10

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DOI： 10.1038/s41428-023-00807-3

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Conjugated photothermal materials and structure design for solar steam generation Invited Reviewed International journal

Chia-Yang Lin, Tsuyoshi Michinobu

Beilstein Journal of Nanotechnology 14 454 - 466 2023.4

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DOI： 10.3762/bjnano.14.36

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Facile access to coil-rod-coil-type block copolymers by CuAAC-based macromolecular clicking

Kosuke Ogita, Naomasa Yomogita, Sultan Otep, Tsuyoshi Michinobu

Polymer Journal 2023.4

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DOI： 10.1038/s41428-022-00714-z

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Cellulose‐based Conductive Gels and Their Applications

Han Jia, Tsuyoshi Michinobu

ChemNanoMat 2023.3

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DOI： 10.1002/cnma.202300020

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Click Synthesis of Triazole Polymers Based on Lignin-Derived Metabolic Intermediate and Their Strong Adhesive Properties to Cu Plate

Yijie Jin, Manjusha Joshi, Takuma Araki, Naofumi Kamimura, Eiji Masai, Masaya Nakamura, Tsuyoshi Michinobu

Polymers 15 ( 6 ) 1349 - 1349 2023.3

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2-Pyrone-4,6-dicarboxylic acid (PDC) is a chemically stable metabolic intermediate of lignin that can be produced on a large scale by transforming bacteria. Novel biomass-based polymers based on PDC were synthesized by Cu(I)-catalyzed azide-alkyne cycloaddition (CuAAC) and fully characterized by nuclear magnetic resonance, infrared spectroscopies, thermal analysis, and tensile lap shear strength measurements. The onset decomposition temperatures of these PDC-based polymers were all above 200 °C. In addition, the PDC-based polymers exhibited strong adhesive properties to various metal plates, with the highest adhesion to a copper plate of 5.73 MPa. Interestingly, this result was in contrast to our previous findings that PDC-based polymers weakly adhere to copper. Furthermore, when bifunctional alkyne and azide monomers were polymerized in situ under hot-press conditions for 1 h, the resulting PDC-based polymer displayed a similar adhesion to a copper plate of 4.18 MPa. The high affinity of the triazole ring to copper ions improved the adhesive ability and selectivity of the PDC-based polymers to copper while still maintaining the strong adhesive ability to other metals, which is conducive to enhancing the versatility of PDC-based polymers as adhesives.

DOI： 10.3390/polym15061349

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Improved supercapacitor performances by adding carbonized C60-based nanospheres to PVA/TEMPO-cellulose hydrogel-based electrolyte

Han Jia, Sabina Shahi, Lok Kumar Shrestha, Katsuhiko Ariga, Tsuyoshi Michinobu

RSC Advances 2023

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DOI： 10.1039/D3RA03349J

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Controlling AIE and ACQ properties of conjugated carbazole-tetraphenylethene copolymers by ethynylene spacer

Han Jia, Ning Xu, Yoshiki Nagai, Marina Doi, Toshiki Sawada, Takeshi Serizawa, Shinji Ando, Satoshi Habuchi, Tsuyoshi Michinobu

Polymer Chemistry 2023

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DOI： 10.1039/D3PY00168G

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Benzothiadiazole versus Thiazolobenzotriazole: A Structural Study of Electron Acceptors in Solution‐Processable Organic Semiconductors Reviewed

Nanami Watanabe, Waner He, Naoya Nozaki, Hidetoshi Matsumoto, Tsuyoshi Michinobu

Chemistry – An Asian Journal 2022.9

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DOI： 10.1002/asia.202200768

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Tuning Ambipolarity of the Conjugated Polymer Channel Layers of Floating-Gate Free Transistors: From Volatile Memories to Artificial Synapses

Yu-Ting Yang, Ying-Sheng Wu, Waner He, Hsin-Chiao Tien, Wei-Chen Yang, Tsuyoshi Michinobu, Wen-Chang Chen, Wen-Ya Lee, Chu-Chen Chueh

ADVANCED SCIENCE 2022.8

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DOI： 10.1002/advs.202203025

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A Route to Conjugated Monomers and Polymers Incorporating 2,5-Connected Oxazole in the Backbone

Joost Kimpel, Waner He, Ye Cheng, Tsuyoshi Michinobu

JOURNAL OF ORGANIC CHEMISTRY 87 ( 14 ) 9384 - 9390 2022.7

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DOI： 10.1021/acs.joc.2c00511

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[2+2] Cycloaddition-retroelectrocyclization reactivity and thin film transistor performances of carbazole-based platinum polyyne polymers

Waner He, Yusuke Washino, Kimie Murata, Naoya Nozaki, Hidetoshi Matsumoto, Tsuyoshi Michinobu

Materials Chemistry and Physics 281 125861 - 125861 2022.4

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DOI： 10.1016/j.matchemphys.2022.125861

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Directional Carrier Polarity Tunability in Ambipolar Organic Transistors Based on Diketopyrrolopyrrole and Bithiophene Imide Dual-Acceptor Semiconducting Polymers

Qian Liu, Waner He, Yongqiang Shi, Sultan Otep, Wen Liang Tan, Sergei Manzhos, Christopher R. McNeill, Xugang Guo, Prashant Sonar, Tsuyoshi Michinobu, Aung Ko Ko Kyaw

CHEMISTRY OF MATERIALS 34 ( 7 ) 3140 - 3151 2022.4

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DOI： 10.1021/acs.chemmater.1c04258

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Postpolymerization Modification: A Powerful Tool for the Synthesis and Function Tuning of Stimuli-Responsive Polymers

Xu Chen, Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 223 ( 1 ) 2022.1

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DOI： 10.1002/macp.202100370

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On-chip silicon-organic hybrid entangled photon pair source

Jinzhao Wang, Yang Wang, Jiewen Li, Rui Li, Yang Feng, Yanmei Li, Jiaxin Chen, Wanxin Li, Yunxu Sun, Yong Yao, Tsuyoshi Michinobu, Xiaochuan Xu

OPTICAL INTERCONNECTS XXII 12007 2022

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DOI： 10.1117/12.2613582

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Structural influences of proquinoidal acceptor moieties on transistor performance and doping capability for diketopyrrolopyrrole-based dual-acceptor conjugated polymers

Ying-Sheng Wu, Jian-Sian Li, Chih-Yuan Chang, Waner He, Tsuyoshi Michinobu, Yan-Cheng Lin, Wen-Chang Chen, Chu-Chen Chueh

Journal of Materials Chemistry C 2022

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DOI： 10.1039/D2TC03956G

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Tetramethylammonium Iodide Additive for Enhancing the Charge Carrier Mobilities of Diketopyrrolopyrrole-Based Conjugated Polymer in Ambipolar Organic Field-Effect Transistors^†

Waner He, Qian Liu, Sultan Otep, Hidetoshi Matsumoto, Sergei Manzhos, Prashant Sonar, Aung Ko Ko Kyaw, Tsuyoshi Michinobu

Chinese Journal of Chemistry 2022

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DOI： 10.1002/cjoc.202200678

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Polyurethanes based on lignin-derived metabolic intermediate with strong adhesion to metals

Ye Cheng, Keiichi Kuboyama, Shuichi Akasaka, Takuma Araki, Eiji Masai, Masaya Nakamura, Tsuyoshi Michinobu

Polymer Chemistry 13 ( 48 ) 6589 - 6598 2022

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Polyurethanes based on lignin-derived 2-pyrone-4,6-dicarboxylic acid (PDC) were successfully synthesized in one-pot, and their thermal, mechanical, and adhesive properties were investigated.

DOI： 10.1039/d2py01128j

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Coil-rod-coil triblock copolymers synthesized by macromolecular clicking and their compatibilizer effects in all-polymer solar cells

Sultan Otep, Yu-Cheng Tseng, Naomasa Yomogita, Jia-Fu Chang, Chu-Chen Chueh, Tsuyoshi Michinobu

JOURNAL OF MATERIALS CHEMISTRY C 10 ( 1 ) 346 - 359 2021.12

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DOI： 10.1039/d1tc04948h

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n-Type Digital Memory Characteristics of Diketopyrrolopyrrole-Based Narrow Bandgap Polymers

Youjin Jung, Wei Li, Jehan Kim, Tsuyoshi Michinobu, Moonhor Ree

JOURNAL OF PHYSICAL CHEMISTRY C 125 ( 49 ) 27479 - 27488 2021.12

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DOI： 10.1021/acs.jpcc.1c08929

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Tuning the Charge Carrier Polarity of Organic Transistors by Varying the Electron Affinity of the Flanked Units in Diketopyrrolopyrrole-Based Copolymers (vol 30, 1907452, 2020)

Qian Liu, Yang Wang, Akihiro Kohara, Hidetoshi Matsumoto, Sergei Manzhos, Krishna Feron, Steven E. Bottle, John Bell, Tsuyoshi Michinobu, Prashant Sonar

ADVANCED FUNCTIONAL MATERIALS 31 ( 37 ) 2021.9

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DOI： 10.1002/adfm.202106250

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Energy-Level Manipulation in Novel Indacenodithiophene-Based Donor-Acceptor Polymers for Near-Infrared Organic Photodetectors

Gurudutt Bhat, Qian Liu, Marcin Kielar, Yuya Hamada, Tsuyoshi Michinobu, Pankaj Sah, Aung Ko Ko Kyaw, Ajay K. Pandey, Prashant Sonar

ACS APPLIED MATERIALS & INTERFACES 13 ( 25 ) 29866 - 29875 2021.6

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DOI： 10.1021/acsami.1c03643

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Cross-Linking of Poly(arylenebutadiynylene)s and Its Effect on Charge Carrier Mobilities in Thin-Film Transistors

Sultan Otep, Kosuke Ogita, Naomasa Yomogita, Kazunori Motai, Yang Wang, Yu-Cheng Tseng, Chu-Chen Chueh, Yuhei Hayamizu, Hidetoshi Matsumoto, Ken Ishikawa, Takehiko Mori, Tsuyoshi Michinobu

MACROMOLECULES 54 ( 9 ) 4351 - 4362 2021.5

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DOI： 10.1021/acs.macromol.1c00008

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Organic J-Aggregate Nanodots with Enhanced Light Absorption and Near-Unity Fluorescence Quantum Yield

Hubert Piwonski, Shuho Nozue, Hiroyuki Fujita, Tsuyoshi Michinobu, Satoshi Habuchi

NANO LETTERS 21 ( 7 ) 2840 - 2847 2021.4

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DOI： 10.1021/acs.nanolett.0c04928

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Conjugated polymers for functional applications: lifetime and performance of polymeric organic semiconductors in organic field-effect transistors

Joost Kimpel, Tsuyoshi Michinobu

POLYMER INTERNATIONAL 70 ( 4 ) 367 - 373 2021.4

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DOI： 10.1002/pi.6020

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Cu(I)-catalyzed azide-alkyne cycloaddition synthesis and fluorescent ion sensor behavior of carbazole-triazole-fluorene conjugated polymers

Shizuka Tane, Tsuyoshi Michinobu

POLYMER INTERNATIONAL 70 ( 4 ) 432 - 436 2021.4

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DOI： 10.1002/pi.5976

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Diketopyrrolopyrrole-thiophene-methoxythiophene based random copolymers for organic field effect transistor applications

Sultan Otep, Yu-Che Lin, Hidetoshi Matsumoto, Takehiko Mori, Kung-Hwa Wei, Tsuyoshi Michinobu

ORGANIC ELECTRONICS 87 2020.12

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DOI： 10.1016/j.orgel.2020.105986

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Millimeter-Deep Detection of Single Shortwave-Infrared-Emitting Polymer Dots through Turbid Media

Hubert Piwonski, Yang Wang, Wei Li, Tsuyoshi Michinobu, Satoshi Habuchi

NANO LETTERS 20 ( 12 ) 8803 - 8810 2020.12

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DOI： 10.1021/acs.nanolett.0c03675

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A cyano-rich small molecule dopant for organic thermoelectrics

Kuan-Heng Tu, Yang Wang, Yasuhiro Kiyota, Takashi Iwahashi, Yukio Ouchi, Takehiko Mori, Tsuyoshi Michinobu

ORGANIC ELECTRONICS 87 105978 - 105978 2020.12

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DOI： 10.1016/j.orgel.2020.105978

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Versatile nature of anthanthrone based polymers as active multifunctional semiconductors for various organic electronic devices

Qian Liu, Yang Wang, Lingeswaran Arunagiri, Muhammad Khatib, Sergei Manzhos, Krishna Feron, Steven E. Bottle, Hossam Haick, He Yan, Tsuyoshi Michinobu, Prashant Sonar

MATERIALS ADVANCES 1 ( 9 ) 3428 - 3438 2020.12

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DOI： 10.1039/d0ma00728e

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Selenium-Based Solar Cell with Conjugated Polymers as Both Electron and Hole Transport Layers to Realize High Water Tolerance as well as Good Long-Term and Thermal Stability

Wenbo Liu, Fei Yu, Yang Wang, Tsuyoshi Michinobu, Weijun Fan, Qichun Zhang

SOLAR RRL 4 ( 12 ) 2020.12

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DOI： 10.1002/solr.202000425

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Poly(3,9-carbazole)s: A Chemically Stable Extended Form of Polyaniline for Nitro-Aromatic Sensor Applications

Joost Kimpel, Yoko Yoshitake, Tsuyoshi Michinobu

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN 93 ( 11 ) 1361 - 1365 2020.11

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DOI： 10.1246/bcsj.20200177

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N-Type Charge Carrier Transport Properties of BDOPV-Benzothiadiazole-Based Semiconducting Polymers

Siyu Wang, Sultan Otep, Joost Kimpel, Takehiko Mori, Tsuyoshi Michinobu

ELECTRONICS 9 ( 10 ) 1604 - 1604 2020.10

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DOI： 10.3390/electronics9101604

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Pure Organic Semiconductor-Based Photoelectrodes for Water Splitting

Sultan Otep, Tsuyoshi Michinobu, Qichun Zhang

SOLAR RRL 4 ( 8 ) 2020.8

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DOI： 10.1002/solr.201900395

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Diketopyrrolopyrrole-Based Dual-Acceptor Copolymers to Realize Tunable Charge Carrier Polarity of Organic Field-Effect Transistors and High-Performance Nonvolatile Ambipolar Flash Memories Reviewed

Qian Liu, Yang Wang, Yi Ren, Akihiro Kohara, Hidetoshi Matsumoto, Yingqian Chen, Sergei Manzhos, Krishna Feron, Steven E. Bottle, John Bell, Ye Zhou, Tsuyoshi Michinobu, Prashant Sonar

ACS Applied Electronic Materials 2 ( 6 ) 1609 - 1618 2020.5

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DOI： 10.1021/acsaelm.0c00169

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Self-Pulsing in Hybrid Subwavelength Grating Metamaterial Ring Resonator

Xiaochuan Xu, Yang Wang, Jiaxin Chen, Wanxin Li, Yaguo Wang, Tsuyoshi Michinobu, Yong Yao, Ray T. Chen

Conference Proceedings - Lasers and Electro-Optics Society Annual Meeting-LEOS 2020- 2020.5

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Development of Block Copolymers with Poly(3-hexylthiophene) Segments as Compatibilizers in Non-Fullerene Organic Solar Cells

Yu-An Su, Noriyuki Maebayashi, Hiroyuki Fujita, Yan-Cheng Lin, Chih- Chen, Wen-Chang Chen, Tsuyoshi Michinobu, Chu-Chen Chueh, Tomoya Higashihara

ACS APPLIED MATERIALS & INTERFACES 12 ( 10 ) 12083 - 12092 2020.3

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DOI： 10.1021/acsami.9b22531

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Improving the air-stability of n-type organic thin-film transistors by polyacrylonitrile additive

Juhong Dong, Yang Wang, Takehiko Mori, Tsuyoshi Michinobu

JAPANESE JOURNAL OF APPLIED PHYSICS 59 2020.3

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DOI： 10.7567/1347-4065/ab5c4b

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Donor-Acceptor Effect of Carbazole-Based Conjugated Polymer Electrets on Photoresponsive Flash Organic Field-Effect Transistor Memories

Chia-Hui Chen, Yang Wang, Tsuyoshi Michinobu, Shu-Wei Chang, Yu-Cheng Chiu, Chun-Yao Ke, Guey-Sheng Liou

ACS APPLIED MATERIALS & INTERFACES 12 ( 5 ) 6144 - 6150 2020.2

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DOI： 10.1021/acsami.9b20960

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Improved Fluorescence and Brightness of Near-Infrared and Shortwave Infrared Emitting Polymer Dots for Bioimaging Applications

Hubert Piwonski, Wei Li, Yang Wang, Tsuyoshi Michinobu, Satoshi Habuchi

ACS APPLIED POLYMER MATERIALS 2 ( 2 ) 569 - 577 2020.2

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DOI： 10.1021/acsapm.9b00967

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Ultrafast Self-Induced Oscillation in a Nonlinear Subwavelength Grating Metamaterial Ring Resonator

Xiaochuan Xu, Yang Wang, Zeyu Pan, Chi-jui Chung, Yue Cheng, Yaguo Wang, Tsuyoshi Michinobu, Ray T. Chen

SILICON PHOTONICS XV 11285 2020

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DOI： 10.1117/12.2544344

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Self-Pulsing in Hybrid Subwavelength Grating Metamaterial Ring Resonator

Xiaochuan Xu, Yang Wang, Jiaxin Chen, Wanxin Li, Yaguo Wang, Tsuyoshi Michinobu, Yong Yao, Ray T. Chen

2020 CONFERENCE ON LASERS AND ELECTRO-OPTICS (CLEO) 2020

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Tuning the Charge Carrier Polarity of Organic Transistors by Varying the Electron Affinity of the Flanked Units in Diketopyrrolopyrrole-Based Copolymers Reviewed

Qian Liu, Yang Wang, Akihiro Kohara, Hidetoshi Matsumoto, Sergei Manzhos, Krishna Feron, Steven E. Bottle, John Bell, Tsuyoshi Michinobu, Prashant Sonar

ADVANCED FUNCTIONAL MATERIALS 30 ( 7 ) 2019.12

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DOI： 10.1002/adfm.201907452

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Energy level tuning of aromatic polyamines by [2+2] cycloaddition-retroelectrocyclization for the optimization of device performances

Kanako Morita, Tsuyoshi Michinobu

SYNTHETIC METALS 257 2019.11

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DOI： 10.1016/j.synthmet.2019.116179

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Novel Photoinduced Recovery of OFET Memories Based on Ambipolar Polymer Electret for Photorecorder Application Reviewed

Chen Chia-Hui, Wang Yang, Tatsumi Hiroki, Michinobu Tsuyoshi, Chang Shu-Wei, Chiu Yu-Cheng, Liou Guey-Sheng

ADVANCED FUNCTIONAL MATERIALS 29 ( 40 ) 2019.10

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DOI： 10.1002/adfm.201902991

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Impact of Incorporating Nitrogen Atoms in Naphthalenediimide-Based Polymer Acceptors on the Charge Generation, Device Performance, and Stability of All-Polymer Solar Cells Reviewed

Sang Woo Kim, Yang Wang, Hoseon You, Wonho Lee, Tsuyoshi Michinobu, Bumjoon J. Kim

ACS Applied Materials & Interfaces 11 ( 39 ) 35896 - 35903 2019.10

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DOI： 10.1021/acsami.9b12037

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Tuning Backbone Planarity in Thiadiazolobenzotriazole-Bis(thienothiophenyl)ethylene Copolymers for Organic Field-Effect Transistors Reviewed

Sultan Otep, Yang Wang, Akihiro Kohara, Hidetoshi Matsumoto, Takehiko Mori, Tsuyoshi Michinobu

ACS APPLIED POLYMER MATERIALS 1 ( 9 ) 2302 - 2312 2019.9

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DOI： 10.1021/acsapm.9b00329

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Significant Difference in Semiconducting Properties of Isomeric All-Acceptor Polymers Synthesized via Direct Arylation Polycondensation Reviewed

Yang Wang, Tsukasa Hasegawa, Hidetoshi Matsumoto, Tsuyoshi Michinobu

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58 ( 34 ) 11893 - 11902 2019.8

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DOI： 10.1002/anie.201904966

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Significant Difference in Semiconducting Properties of Isomeric All-Acceptor Polymers Synthesized via Direct Arylation Polycondensation Reviewed

Yang Wang, Tsukasa Hasegawa, Hidetoshi Matsumoto, Tsuyoshi Michinobu

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58 ( 34 ) 11893 - 11902 2019.8

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DOI： 10.1002/anie.201904966

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Efficient Inverted Perovskite Solar Cells by Employing N-Type (D-A(1)-D-A(2)) Polymers as Electron Transporting Layer Reviewed

Said Ahmed Ali, Xie Jian, Wang Yang, Wang Zongrui, Zhou Yu, Zhao Kexiang, Gao Wei-Bo, Michinobu Tsuyoshi, Zhang Qichun

SMALL 15 ( 29 ) 2019.7

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DOI： 10.1002/smll.201803339

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Elucidating the thermal degradation of carbazole-containing platinum-polyyne polymers Reviewed

Lisa Gabriela, Yoshitake Yoko, Michinobu Tsuyoshi

JOURNAL OF APPLIED POLYMER SCIENCE 136 ( 24 ) 2019.6

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DOI： 10.1002/app.47639

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Dual Imide-Functionalized Unit-Based Regioregular D-A(1)-D-A(2) Polymers for Efficient Unipolar n-Channel Organic Transistors and All-Polymer Solar Cells Reviewed

Yang Wang, Sang Woo Kim, Junbok Lee, Hidetoshi Matsumoto, Bumjoon J. Kim, Tsuyoshi Michinobu

ACS APPLIED MATERIALS & INTERFACES 11 ( 25 ) 22583 - 22594 2019.6

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DOI： 10.1021/acsami.9b05537

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Poly(dithiazolfluorene-alt-selenadiazolobenzotriazole)-Based Blue-Light Photodetector and Its Application in Visible-Light Communication Reviewed

Hang Guo, Yang Wang, Rui Wang, Shengze Liu, Kai Huang, Tsuyoshi Michinobu, Guifang Dong

ACS Applied Materials & Interfaces 11 ( 18 ) 16758 - 16764 2019.5

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DOI： 10.1021/acsami.9b00467

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Strain‐Promoted Double Azide Addition to Octadehydrodibenzo[12]annulene Derivatives Reviewed

Satomi Fukushima, Minoru Ashizawa, Susumu Kawauchi, Tsuyoshi Michinobu

Helvetica Chimica Acta 102 ( 4 ) e1900016 2019.4

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DOI： 10.1002/hlca.201900016

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Significant Improvement of Unipolar n-Type Transistor Performances by Manipulating the Coplanar Backbone Conformation of Electron-Deficient Polymers via Hydrogen Bonding Reviewed

Yang Wang, Tsukasa Hasegawa, Hidetoshi Matsumoto, Tsuyoshi Michinobu

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 141 ( 8 ) 3566 - 3575 2019.2

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DOI： 10.1021/jacs.8b12499

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Development of N-Type Semiconducting Polymers for Transistor Applications Reviewed

Michinobu Tsuyoshi

JOURNAL OF PHOTOPOLYMER SCIENCE AND TECHNOLOGY 32 ( 4 ) 563 - 570 2019

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DOI： 10.2494/photopolymer.32.563

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Antibacterial Polymeric Films Fabricated by [2+2] Cycloaddition–Retroelectrocyclization and Ag + Ion Coordination Reviewed

Hiroyuki Fujita, Nahoko Nihei, Masami Bito, Tsuyoshi Michinobu

Macromolecular Bioscience 18 ( 12 ) 1800336 - 1800336 2018.12

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Covalent layer-by-layer thin films with charge-transfer chromophores: side chain engineering for efficient Ag+ ion recognition in aqueous solutions Reviewed

Fujita Hiroyuki, Michinobu Tsuyoshi

SOFT MATTER 14 ( 44 ) 9055 - 9060 2018.11

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A Direct Method to Access Substituted Pyreno[4,5-c:9,10-c '(]) difuran and its Analogues Reviewed

Chen Wangqiao, Long Guankui, Kanehira Koji, Zhang Mingtao, Michinobu Tsuyoshi, Liu Ming, Zhang Qichun

ASIAN JOURNAL OF ORGANIC CHEMISTRY 7 ( 11 ) 2213 - 2217 2018.11

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Rational design strategies for electron-deficient semiconducting polymers in ambipolar/n-channel organic transistors and all-polymer solar cells Reviewed

Wang Yang, Michinobu Tsuyoshi

JOURNAL OF MATERIALS CHEMISTRY C 6 ( 39 ) 10390 - 10410 2018.10

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Well-designed dopamine-imprinted polymer interface for selective and quantitative dopamine detection among catecholamines using a potentiometric biosensor. Reviewed International journal

Taira Kajisa, Wei Li, Tsuyoshi Michinobu, Toshiya Sakata

Biosensors & bioelectronics 117 810 - 817 2018.10

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DOI： 10.1016/j.bios.2018.07.014

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Perovskite solar cells based on hole-transporting conjugated polymers by direct arylation polycondensation Reviewed

Wei Li, Takehiko Mori, Tsuyoshi Michinobu

MRS Communications 8 ( 3 ) 1 - 1253 2018.7

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DOI： 10.1557/mrc.2018.119

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Catecholamine Detection Using a Functionalized Poly(l-dopa)-Coated Gate Field-Effect Transistor. Reviewed International journal

Taira Kajisa, Wei Li, Tsuyoshi Michinobu

ACS omega 3 ( 6 ) 6719 - 6727 2018.6

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DOI： 10.1021/acsomega.8b00518

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Functional Covalent Layer-by-Layer Thin Films by [2 + 2] Cycloaddition-Retroelectrocyclization Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu

ACS Macro Letters 7 ( 6 ) 716 - 719 2018.6

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DOI： 10.1021/acsmacrolett.8b00365

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The [2+2] Cycloaddition-Retroelectrocyclization (CA-RE) Click Reaction: Facile Access to Molecular and Polymeric Push-Pull Chromophores Reviewed

Tsuyoshi Michinobu, François Diederich

Angewandte Chemie - International Edition 57 ( 14 ) 3552 - 3577 2018.3

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DOI： 10.1002/anie.201711605

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High-Performance n-Channel Organic Transistors Using High-Molecular-Weight Electron-Deficient Copolymers and Amine-Tailed Self-Assembled Monolayers Reviewed

Yang Wang, Tsukasa Hasegawa, Hidetoshi Matsumoto, Takehiko Mori, Tsuyoshi Michinobu

ADVANCED MATERIALS 30 ( 13 ) 1707164 2018.3

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DOI： 10.1002/adma.201707164

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Die [2+2]-Cycloadditions-Retroelektrocyclisierungs(CA-RE)-Klick-Reaktion: ein einfacher Zugang zu molekularen und polymeren Push-pull-Chromophoren Reviewed

Tsuyoshi Michinobu, Fran{\c{c } }ois Diederich

Angewandte Chemie 130 ( 14 ) 3612 - 3638 2018.3

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Temperature compensation of pressure-sensitive luminescent polymer sensors Reviewed

Sachiko Sano, Takahiro Yuuki, Tsuyoshi Hyakutake, Katsuaki Morita, Hirotaka Sakaue, Satoshi Arai, Hidetoshi Matsumoto, Tsuyoshi Michinobu

SENSORS AND ACTUATORS B-CHEMICAL 255 1960 - 1966 2018.2

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Highly-stable, green-solvent-processable organic thin-film transistors: Angular-: vs. linear-shaped carbazoledioxazine derivatives Reviewed

Yang Wang, Hiroki Tatsumi, Rikuo Otsuka, Takehiko Mori, Tsuyoshi Michinobu

Journal of Materials Chemistry C 6 ( 22 ) 5865 - 5876 2018

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DOI： 10.1039/c8tc01711e

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Highly-stable, green-solvent-processable organic thin-film transistors: Angular-: vs. linear-shaped carbazoledioxazine derivatives Reviewed

Yang Wang, Hiroki Tatsumi, Rikuo Otsuka, Takehiko Mori, Tsuyoshi Michinobu

Journal of Materials Chemistry C 6 ( 22 ) 5865 - 5876 2018

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Linear-type carbazoledioxazine-based organic semiconductors: The effect of backbone planarity on the molecular orientation and charge transport properties Reviewed

Rikuo Otsuka, Yang Wang, Takehiko Mori, Tsuyoshi Michinobu

RSC Advances 8 ( 18 ) 9822 - 9832 2018

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DOI： 10.1039/c8ra01088a

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Inversion of charge carrier polarity and boosting the mobility of organic semiconducting polymers based on benzobisthiadiazole derivatives by fluorination Reviewed

Yang Wang, Aaron Tze-Rue Tan, Takehiko Mori, Tsuyoshi Michinobu

Journal of Materials Chemistry C 6 ( 14 ) 3593 - 3603 2018

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DOI： 10.1039/c7tc04993e

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Rational design strategies for electron-deficient semiconducting polymers in ambipolar/n-channel organic transistors and all-polymer solar cells Reviewed

Yang Wang, Tsuyoshi Michinobu

Journal of Materials Chemistry C 2018

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DOI： 10.1039/C8TC03967D

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Covalent layer-by-layer thin films with charge-transfer chromophores: side chain engineering for efficient Ag+ ion recognition in aqueous solutions Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu

Soft Matter 2018

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DOI： 10.1039/C8SM01986J

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Linear-type carbazoledioxazine-based organic semiconductors: The effect of backbone planarity on the molecular orientation and charge transport properties Reviewed

Rikuo Otsuka, Yang Wang, Takehiko Mori, Tsuyoshi Michinobu

RSC Advances 8 ( 18 ) 9822 - 9832 2018

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DOI： 10.1039/c8ra01088a

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Inversion of charge carrier polarity and boosting the mobility of organic semiconducting polymers based on benzobisthiadiazole derivatives by fluorination Reviewed

Yang Wang, Aaron Tze-Rue Tan, Takehiko Mori, Tsuyoshi Michinobu

Journal of Materials Chemistry C 6 ( 14 ) 3593 - 3603 2018

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DOI： 10.1039/c7tc04993e

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Polymeric Chemosensors: A Conventional Platform with New Click Chemistry Reviewed

Yang Wang, Tsuyoshi Michinobu

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN 90 ( 12 ) 1388 - 1400 2017.12

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DOI： 10.1246/bcsj.20170294

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D-A(1)-D-A(2) Backbone Strategy for Benzobisthiadiazole Based n-Channel Organic Transistors: Clarifying the Selenium-Substitution Effect on the Molecular Packing and Charge Transport Properties in Electron-Deficient Polymers Reviewed

Yang Wang, Tsukasa Hasegawa, Hidetoshi Matsumoto, Takehiko Mori, Tsuyoshi Michinobu

ADVANCED FUNCTIONAL MATERIALS 27 ( 33 ) 2017.9

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DOI： 10.1002/adfm.201701486

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Polarity Engineering of Benzobisthiadiazole-Based Polymer Thin Film Transistors by Variation of Electron Affinity of the Comonomers Reviewed

Yang Wang, Ryuhei Hosokawa, Takehiko Mori, Tsuyoshi Michinobu

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN 90 ( 9 ) 1041 - 1049 2017.9

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DOI： 10.1246/bcsj.20170158

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Colorimetric Ion Sensors Based on Polystyrenes Bearing Side Chain Triazole and Donor-Acceptor Chromophores Reviewed

Yongrong Li, Yusuke Washino, Tsuyoshi Hyakutake, Tsuyoshi Michinobu

ANALYTICAL SCIENCES 33 ( 5 ) 599 - 604 2017.5

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Controlling photophysical properties of ultrasmall conjugated polymer nanoparticles through polymer chain packing Reviewed

Hubert Piwonski, Tsuyoshi Michinobu, Satoshi Habuchi

NATURE COMMUNICATIONS 8 2017.5

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Side-Chain Engineering of Polyphenylacetylene Derivatives for Tuning the Self-Assembly and Gas Permeability Properties Reviewed

Yongrong Li, Hiroyuki Fujita, Tsuyoshi Hyakutake, Tsuyoshi Michinobu

JOURNAL OF FIBER SCIENCE AND TECHNOLOGY 73 ( 4 ) 82 - 86 2017.4

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Naphthodithiophenediimide-Benzobisthiadiazole-Based Polymers: Versatile n-Type Materials for Field-Effect Transistors and Thermoelectric Devices Reviewed

Yang Wang, Masahiro Nakano, Tsuyoshi Michinobu, Yasuhiro Kiyota, Takehiko Mori, Kazuo Takimiya

MACROMOLECULES 50 ( 3 ) 857 - 864 2017.2

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Rational Design of High-Mobility Semicrystalline Conjugated Polymers with Tunable Charge Polarity: Beyond Benzobisthiadiazole-Based Polymers Reviewed

Yang Wang, Tsukasa Hasegawa, Hidetoshi Matsumoto, Takehiko Mori, Tsuyoshi Michinobu

ADVANCED FUNCTIONAL MATERIALS 27 ( 2 ) 2017.1

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Electrochromic Behavior of Donor-Acceptor Polymers Containing Diketopyrrolopyrrole Unit Reviewed

Wei Li, Tsuyoshi Michinobu

JOURNAL OF PHOTOPOLYMER SCIENCE AND TECHNOLOGY 30 ( 4 ) 495 - 499 2017

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Halogen Substitution Effects on the Molecular Packing and Thin Film Transistor Performances of Carbazoledioxazine Derivatives Reviewed

Hiroki Tatsumi, Yang Wang, Yosuke Aizawa, Masatoshi Tokita, Takehiko Mori, Tsuyoshi Michinobu

Journal of Physical Chemistry C 120 ( 47 ) 26686 - 26694 2016.12

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DOI： 10.1021/acs.jpcc.6b09888

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Novel Design of Carbazole-Based Donor-Acceptor Molecules for Fullerene-Free Organic Photovoltaic Devices Reviewed

Tsuyoshi Michinobu, Naoya Yamada, Yusuke Washino, Ken-ichi Nakayama

JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY 16 ( 8 ) 8662 - 8669 2016.8

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Thermal degradation of some ferrocene-containing poly(aryleneethynylene)s Reviewed

Gabriela Lisa, Yoko Yoshitake, Tsuyoshi Michinobu

JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS 120 399 - 408 2016.7

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3,6-Carbazole vs 2,7-carbazole: A comparative study of hole-transporting polymeric materials for inorganic-organic hybrid perovskite solar cells Reviewed

Wei Li, Munechika Otsuka, Takehito Kato, Yang Wang, Takehiko Mori, Tsuyoshi Michinobu

BEILSTEIN JOURNAL OF ORGANIC CHEMISTRY 12 1401 - 1409 2016.7

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Troger's Base-Containing Aromatic Polymers with Unexpected Properties Endowed by the Insertion of Alkyne Spacers Reviewed

Wei Li, Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 217 ( 7 ) 863 - 870 2016.4

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DOI： 10.1002/macp.201500494

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Sequentially Different AB Diblock and ABA Triblock Copolymers as P3HT:PCBM Interfacial Compatibilizers for Bulk-Heterojunction Photovoltaics Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu, Seijiro Fukuta, Tomoyuki Koganezawa, Tomoya Higashihara

ACS APPLIED MATERIALS & INTERFACES 8 ( 8 ) 5484 - 5492 2016.3

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Cross-linking and postfunctionalization of polymer films by utilizing the orthogonal reactivity of 7,7,8,8-tetracyanoquinodimethane Reviewed

Yusuke Washino, Tsuyoshi Michinobu

PHYSICAL CHEMISTRY CHEMICAL PHYSICS 18 ( 4 ) 2288 - 2291 2016.1

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Synthesis of novel polymeric energy materials with high nitrogen content by double click functionalization Reviewed

Tsuyoshi Michinobu, Yoko Yoshitake

SCIENCE AND TECHNOLOGY OF ENERGETIC MATERIALS 77 ( 3-4 ) 86 - 90 2016

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Synthesis of Fullerene Polymers and Preparation of Electrospun Microfibers Thereof Reviewed

Tsuyoshi Michinobu, Kimie Murata, Hidetoshi Matsumoto

KOBUNSHI RONBUNSHU 73 ( 3 ) 258 - 261 2016

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Benzothiadiazole and its pi-extended, heteroannulated derivatives: useful acceptor building blocks for high-performance donor-acceptor polymers in organic electronics Reviewed

Yang Wang, Tsuyoshi Michinobu

JOURNAL OF MATERIALS CHEMISTRY C 4 ( 26 ) 6200 - 6214 2016

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Structural effects of dibromocarbazoles on direct arylation polycondensation with 3,4-ethylenedioxythiophene Reviewed

Wei Li, Tsuyoshi Michinobu

POLYMER CHEMISTRY 7 ( 18 ) 3165 - 3171 2016

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DOI： 10.1039/c6py00381h

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High-performance triazole-containing brush polymers via azide-alkyne click chemistry: a new functional polymer platform for electrical memory devices Reviewed

Sungjin Song, Yong-Gi Ko, Hoyeol Lee, Dongwoo Wi, Brian J. Ree, Yongrong Li, Tsuyoshi Michinobu, Moonhor Ree

NPG ASIA MATERIALS 7 2015.12

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DOI： 10.1038/am.2015.130

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Efficient Synthesis and Photosensitizer Performance of Nonplanar Organic Donor-Acceptor Molecules Reviewed

Yuping Yuan, Tsuyoshi Michinobu, Norifusa Satoh, Minoru Ashizawa, Liyuan Han

JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY 15 ( 8 ) 5856 - 5866 2015.8

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Click Functionalization of Aromatic Polymers for Organic Electronic Device Applications Reviewed

Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 216 ( 13 ) 1387 - 1395 2015.7

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DOI： 10.1002/macp.201500086

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New Semiconducting Polymers Based on Benzobisthiadiazole Analogues: Tuning of Charge Polarity in Thin Film Transistors via Heteroatom Substitution Reviewed

Yang Wang, Hiroyasu Masunaga, Takaaki Hikima, Hidetoshi Matsumoto, Takehiko Mori, Tsuyoshi Michinobu

MACROMOLECULES 48 ( 12 ) 4012 - 4023 2015.6

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Synthesis and Photovoltaic Properties of Thieno[3,4-b]pyrazine or Dithieno[3 ',2 ':3,4;2 '',3 '':5,6]benzo[1,2-d]imidazole-Containing Conjugated Polymers Reviewed

Mukhamed L. Keshtov, Dmitri Yu. Godovsky, Alexei R. Khokhlov, Tetsunari Mizobe, Hiroyuki Fujita, Eisuke Goto, Junya Hiyoshi, Saki Nakamura, Susumu Kawauchi, Tomoya Higashihara, Tsuyoshi Michinobu

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY 53 ( 9 ) 1067 - 1075 2015.5

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DOI： 10.1002/pola.27570

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Reversible Transformation of a One-Handed Helical Foldamer Utilizing a Planarity-Switchable Spacer and C-2-Chiral Spirobifluorene Units Reviewed

Hitoshi Okuda, Yasuhito Koyama, Satoshi Uchida, Tsuyoshi Michinobu, Hiromitsu Sogawa, Toshikazu Takata

ACS Macro Letters 4 ( 4 ) 462 - 466 2015.4

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DOI： 10.1021/acsmacrolett.5b00176

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Bulk-Heterojunction Organic Solar Cells Based on Benzobisthiadiazole Semiconducting Polymers Reviewed

Yang Wang, Michael F. G. Klein, Junya Hiyoshi, Susumu Kawauchi, Wallace W. H. Wong, Tsuyoshi Michinobu

JOURNAL OF PHOTOPOLYMER SCIENCE AND TECHNOLOGY 28 ( 3 ) 385 - 391 2015

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DOI： 10.2494/photopolymer.28.385

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Benzobisthiadiazole-based conjugated dono-racceptor polymers for organic thin film transistors: effects of pi-conjugated bridges on ambipolar transport Reviewed

Yang Wang, Tomofumi Kadoya, Lei Wang, Teruaki Hayakawa, Masatoshi Tokita, Takehiko Mori, Tsuyoshi Michinobu

JOURNAL OF MATERIALS CHEMISTRY C 3 ( 6 ) 1196 - 1207 2015

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DOI： 10.1039/c4tc02273d

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New Fullerene-Based Polymers and Their Electrical Memory Characteristics Reviewed

Yong-Gi Ko, Suk Gyu Hahm, Kimie Murata, Young Yong Kim, Brian J. Ree, Sungjin Song, Tsuyoshi Michinobu, Moonhor Ree

MACROMOLECULES 47 ( 23 ) 8154 - 8163 2014.12

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DOI： 10.1021/ma5021402

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STEPWISE SYNTHESES OF 3,6-CARBAZOLE-BASED CONJUGATED OLIGOMERS Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu

HETEROCYCLES 89 ( 10 ) 2346 - 2355 2014.10

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DOI： 10.3987/COM-14-13080

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Sequence-Regulated Linear Polymers with Ion-Sensing Charge-Transfer Chromophores by the Multiple Click Approach Reviewed

Yusuke Washino, Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 215 ( 15 ) 1485 - 1490 2014.8

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DOI： 10.1002/macp.201400275

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Digital Memory Versatility of Fully pi-Conjugated Donor-Acceptor Hybrid Polymers Reviewed

Yong-Gi Ko, Dong Min Kim, Kyungtae Kim, Sungmin Jung, Dongwoo Wi, Tsuyoshi Michinobu, Moonhor Ree

ACS APPLIED MATERIALS & INTERFACES 6 ( 11 ) 8415 - 8425 2014.6

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DOI： 10.1021/am5013134

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Novel design of organic donor-acceptor dyes without carboxylic acid anchoring groups for dye-sensitized solar cells Reviewed

Tsuyoshi Michinobu, Norifusa Satoh, Jinhua Cai, Yongrong Li, Liyuan Han

JOURNAL OF MATERIALS CHEMISTRY C 2 ( 17 ) 3367 - 3372 2014

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DOI： 10.1039/c3tc32165g

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Attempted Inversion of Semiconducting Features of Platinum Polyyne Polymers: A New Approach for All-Polymer Solar Cells Reviewed

Yuping Yuan, Tsuyoshi Michinobu, Jun Oguma, Takehito Kato, Kunihito Miyake

MACROMOLECULAR CHEMISTRY AND PHYSICS 214 ( 13 ) 1465 - 1472 2013.7

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DOI： 10.1002/macp.201300245

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Structural Requirements for Producing Solvent-Free Room Temperature Liquid Fullerenes Reviewed

Tsuyoshi Michinobu, Kensuke Okoshi, Yoshihiko Murakami, Kiyotaka Shigehara, Katsuhiko Ariga, Takashi Nakanishi

LANGMUIR 29 ( 17 ) 5337 - 5344 2013.4

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DOI： 10.1021/la400969f

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Polymeric ion sensors with multiple detection modes achieved by a new type of click chemistry reaction Reviewed

Tsuyoshi Michinobu, Yongrong Li, Tsuyoshi Hyakutake

Physical Chemistry Chemical Physics 15 ( 8 ) 2623 - 2631 2013.2

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DOI： 10.1039/c2cp43203j

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Sequential and click-type postfunctionalization of regioregular poly(3-hexylthiophene) for realization of n-doped multiplet state Reviewed

Yuping Yuan, Wonsung Choi, Hiroyuki Nishide, Tsuyoshi Michinobu

CHEMICAL SCIENCE 4 ( 1 ) 345 - 350 2013

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DOI： 10.1039/c2sc21334f

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Synthesis and Postfunctionalization of Rod-Coil Diblock and Coil-Rod-Coil Triblock Copolymers Composed of Poly(3-hexylthiophene) and Poly(4-(4 '-N,N-dihexylaminophenylethynyl)styrene) Segments Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu, Masatoshi Tokita, Mitsuru Ueda, Tomoya Higashihara

MACROMOLECULES 45 ( 24 ) 9643 - 9656 2012.12

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DOI： 10.1021/ma301692b

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Construction of Donor-Acceptor Chromophores in Platinum Polyyne Polymer by [2+2] Cycloaddition of Organic Acceptors Reviewed

Yuping Yuan, Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 213 ( 20 ) 2114 - 2119 2012.10

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DOI： 10.1002/macp.201200316

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Covalently bonded layer-by-layer films by high-yielding addition reaction between electron-rich alkynes and tetracyanoquinodimethane Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu

ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY 244 2012.8

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Click synthesis of low band gap semiconducting polymers Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu

ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY 244 2012.8

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Postfunctionalization of aromatic polyamine by [2+2] cycloaddition of 7,7,8,8-tetracyanoquinodimethane with side chain alkynes Reviewed

Yusuke Washino, Kimie Murata, Tsuyoshi Michinobu

POLYMER BULLETIN 69 ( 2 ) 137 - 147 2012.7

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DOI： 10.1007/s00289-011-0693-7

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Click Synthesis and Reversible Electrochromic Behaviors of Novel Polystyrenes Bearing Aromatic Amine Units Reviewed

Yongrong Li, Tsuyoshi Michinobu

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY 50 ( 11 ) 2111 - 2120 2012.6

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DOI： 10.1002/pola.25990

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Synthesis and Photovoltaic Properties of 1,8-Carbazole-Based Donor-Acceptor Type Conjugated Polymers Reviewed

Hiroyuki Fujita, Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 213 ( 4 ) 447 - 457 2012.2

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DOI： 10.1002/macp.201100591

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Colorimetric sensing of cations and anions by clicked polystyrenes bearing side chain donor-acceptor chromophores Reviewed

Yongrong Li, Minoru Ashizawa, Satoshi Uchida, Tsuyoshi Michinobu

POLYMER CHEMISTRY 3 ( 8 ) 1996 - 2005 2012

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DOI： 10.1039/c2py20230a

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Multi-coloration of polyurethane derivatives through click postfunctionalization, electrochemical oxidation, and Ag+ ion complexation Reviewed

Yongrong Li, Tsuyoshi Michinobu

JOURNAL OF MATERIALS CHEMISTRY 22 ( 19 ) 9513 - 9521 2012

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DOI： 10.1039/c2jm30298e

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Emergence of Colorimetric Chemosensor Ability of Metal Ions in TCNQ Polyester by Postfunctionalization Reviewed

Yusuke Washino, Tsuyoshi Michinobu

JOURNAL OF PHOTOPOLYMER SCIENCE AND TECHNOLOGY 25 ( 3 ) 267 - 270 2012

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DOI： 10.2494/photopolymer.25.267

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Effects of click postfunctionalization on thermal stability and field effect transistor performances of aromatic polyamines Reviewed

Tsuyoshi Michinobu, Chayeon Seo, Keiichi Noguchi, Takehiko Mori

POLYMER CHEMISTRY 3 ( 6 ) 1427 - 1435 2012

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DOI： 10.1039/c2py20079a

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Twist Angle Plays an Important Role in Photophysical Properties of a Donor-Acceptor-Type Conjugated Polymer: A Combined Ensemble and Single-Molecule Study Reviewed

Satoshi Habuchi, Hiroyuki Fujita, Tsuyoshi Michinobu, Martin Vacha

JOURNAL OF PHYSICAL CHEMISTRY B 115 ( 49 ) 14404 - 14415 2011.12

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DOI： 10.1021/jp209405k

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A Novel Polymeric Chemosensor: Dual Colorimetric Detection of Metal Ions Through Click Synthesis Reviewed

Yongrong Li, Minoru Ashizawa, Satoshi Uchida, Tsuyoshi Michinobu

MACROMOLECULAR RAPID COMMUNICATIONS 32 ( 22 ) 1804 - 1808 2011.11

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DOI： 10.1002/marc.201100397

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Multicolor emission and thin film transistor properties of 1,8-diethynylcarbazole-based conjugated copolymers Reviewed

Tsuyoshi Michinobu, Haruka Osako, Chayeon Seo, Kimie Murata, Takehiko Mori, Kiyotaka Shigehara

POLYMER 52 ( 25 ) 5756 - 5763 2011.11

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DOI： 10.1016/j.polymer.2011.10.028

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Electrical Memory Characteristics of Nitrogen-Linked Poly(2,7-carbazole)s Reviewed

Suk Gyu Hahm, Taek Joon Lee, Dong Min Kim, Wonsang Kwon, Yong-Gi Ko, Tsuyoshi Michinobu, Moonhor Ree

JOURNAL OF PHYSICAL CHEMISTRY C 115 ( 44 ) 21954 - 21962 2011.11

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DOI： 10.1021/jp207211e

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Origin of Second-Order Nonlinear Optical Effects of Nonpoled Donor-Acceptor Chromophores on Surface Reviewed

Tsuyoshi Michinobu, Yongrong Li, Yusuke Washino, Kimie Murata, Kazuma Tsuboi

JAPANESE JOURNAL OF APPLIED PHYSICS 50 ( 9 ) 2011.9

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DOI： 10.1143/JJAP.50.09MA06

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High-Yielding Alkyne-Tetracyanoethylene Addition Reactions: A Powerful Tool for Analyzing Alkyne-Linked Conjugated Polymer Structures Reviewed

Hiroyuki Fujita, Kazuma Tsuboi, Tsuyoshi Michinobu

MACROMOLECULAR CHEMISTRY AND PHYSICS 212 ( 16 ) 1758 - 1766 2011.8

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DOI： 10.1002/macp.201100198

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Oxygen permeability control of polyphenylacetylene derivatives by postfunctionalization using alkyne-TCNE click chemistry Reviewed

Yongrong Li, Tsuyoshi Hyakutake, Tsuyoshi Michinobu

ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY 242 2011.8

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Click synthesis and adhesive properties of novel biomass-based polymers from lignin-derived stable metabolic intermediate Reviewed

Tsuyoshi Michinobu, Kenta Hiraki, Yasunori Inazawa, Yoshihiro Katayama, Eiji Masai, Masaya Nakamura, Seiji Ohara, Kiyotaka Shigehara

POLYMER JOURNAL 43 ( 7 ) 648 - 653 2011.7

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DOI： 10.1038/pj.2011.40

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Oxygen Permeability Change of Polyphenylacetylene Derivatives by Postfunctional TCNE Addition Reviewed

Yongrong Li, Tsuyoshi Hyakutake, Tsuyoshi Michinobu

CHEMISTRY LETTERS 40 ( 6 ) 570 - 572 2011.6

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DOI： 10.1246/cl.2011.570

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Liquid Crystallinity and Organogelation Behavior of Lignin-Derived Metabolic Intermediate Bearing Cholesterol Groups Reviewed

Tsuyoshi Michinobu, Kenta Hiraki, Nozomu Fujii, Kazuhiro Shikinaka, Yoshihiro Katayama, Eiji Masai, Masaya Nakamura, Yuichiro Otsuka, Seiji Ohara, Kiyotaka Shigehara

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN 84 ( 6 ) 667 - 674 2011.6

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DOI： 10.1246/bcsj.20110055

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Creation of persistent charge-transfer interactions in TCNQ polyester Reviewed

Yusuke Washino, Kimie Murata, Minoru Ashizawa, Susumu Kawauchi, Tsuyoshi Michinobu

POLYMER JOURNAL 43 ( 4 ) 364 - 369 2011.4

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DOI： 10.1038/pj.2011.2

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Application of Alkyne-TCNQ Addition Reaction to Polymerization Reviewed

Yusuke Washino, Tsuyoshi Michinobu

MACROMOLECULAR RAPID COMMUNICATIONS 32 ( 8 ) 644 - 648 2011.4

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DOI： 10.1002/marc.201100025

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Microwave-Assisted TCNE/TCNQ Addition to Poly(thienyleneethynylene) Derivative for Construction of Donor-Acceptor Chromophores Reviewed

Yuping Yuan, Tsuyoshi Michinobu, Minoru Ashizawa, Takehiko Mori

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY 49 ( 4 ) 1013 - 1020 2011.2

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DOI： 10.1002/pola.24515

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One-Step Synthesis of Ladder-Type Fused Poly(benzopentalene) Derivatives with Tunable Energy Levels by Variable Substituents Reviewed

Dong Wang, Tsuyoshi Michinobu

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY 49 ( 1 ) 72 - 81 2011.1

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DOI： 10.1002/pola.24419

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Energy Level Tuning of Polythiophene Derivative by Click Chemistry-Type Postfunctionalization of Side-Chain Alkynes Reviewed

Yuping Yuan, Tsuyoshi Michinobu

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY 49 ( 1 ) 225 - 233 2011.1

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DOI： 10.1002/pola.24443

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Photochemical control of a highly efficient addition reaction between electron-rich alkynes and tetracyanoethylene Reviewed

Masakazu Morimoto, Kimie Murata, Tsuyoshi Michinobu

CHEMICAL COMMUNICATIONS 47 ( 35 ) 9819 - 9821 2011

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DOI： 10.1039/c1cc13476k

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Simultaneous Formation of Donor-acceptor Chromophores and Cross-linking for Electro-optic Polymer Materials Reviewed

Yusuke Washino, Kazuma Tsuboi, Tsuyoshi Michinobu

JOURNAL OF PHOTOPOLYMER SCIENCE AND TECHNOLOGY 24 ( 3 ) 305 - 309 2011

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DOI： 10.2494/photopolymer.24.305

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Photochromism of Azopyridine Side Chain Polymer Controlled by Supramolecular Self-Assembly Reviewed

Tsuyoshi Michinobu, Rinako Eto, Hiroe Kumazawa, Nozomu Fujii, Kiyotaka Shigehara

JOURNAL OF MACROMOLECULAR SCIENCE PART A-PURE AND APPLIED CHEMISTRY 48 ( 8 ) 625 - 631 2011

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DOI： 10.1080/15226514.2011.586279

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Photochromic Behaviors of N-Isopropylacrylamide Copolymers Containing Azopyridine-Dyes Reviewed

Tsuyoshi Michinobu, Rinako Eto, Kiyotaka Shigehara

KOBUNSHI RONBUNSHU 68 ( 4 ) 195 - 197 2011

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DOI： 10.1295/koron.68.195

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Langmuir monolayers of a cholesterol-armed cyclen complex that can control enantioselectivity of amino acid recognition by surface pressure Reviewed

Tsuyoshi Michinobu, Satoshi Shinoda, Takashi Nakanishi, Jonathan P. Hill, Kazuko Fujii, Tomoko N. Player, Hiroshi Tsukube, Katsuhiko Ariga

PHYSICAL CHEMISTRY CHEMICAL PHYSICS 13 ( 11 ) 4895 - 4900 2011

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DOI： 10.1039/c0cp01990a

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F(4)TCNQ Doping of P3HT:PCBM Photovoltaic Devices Reviewed

Hiroyuki Fujita, Yuping Yuan, Tsuyoshi Michinobu

JOURNAL OF PHOTOPOLYMER SCIENCE AND TECHNOLOGY 24 ( 3 ) 311 - 315 2011

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DOI： 10.2494/photopolymer.24.311

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Adapting semiconducting polymer doping techniques to create new types of click postfunctionalization Reviewed

Tsuyoshi Michinobu

CHEMICAL SOCIETY REVIEWS 40 ( 5 ) 2306 - 2316 2011

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DOI： 10.1039/c0cs00205d

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Postfunctionalization of Alkyne-Linked Conjugated Carbazole Polymer by Thermal Addition Reaction of Tetracyanoethylene Reviewed

Tsuyoshi Michinobu, Hiroyuki Fujita

MATERIALS 3 ( 10 ) 4773 - 4783 2010.10

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DOI： 10.3390/ma3104773

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Efficient Synthesis of Block Copolymers Bearing Donor-Acceptor Chromophores for Second-Order Nonlinear Optical Applications

Li, Yongrong, Tsuboi, Kazuma, Michinobu, Tsuyoshi, Ishida, Yoshihito, Hirai, Tomoyasu, Hayakawa, Teruaki, Kakimoto, Masa-aki

Journal of Photopolymer Science and Technology 23 ( 3 ) 2010

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DOI： 10.2494/photopolymer.23.337

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Double Click Synthesis and Second-Order Nonlinearities of Polystyrenes Bearing Donor-Acceptor Chromophores

Li, Yongrong, Tsuboi, Kazuma, Michinobu, Tsuyoshi

Macromolecules 43 ( 12 ) 2010

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DOI： 10.1021/ma100869m

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Click synthesis of donor-acceptor-type aromatic polymers

Michinobu, Tsuyoshi

Pure and Applied Chemistry 82 ( 4 ) 2010

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DOI： 10.1351/PAC-CON-09-09-09

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Blue, Green, and Red Light Emission of 1,8-Carbazole-based Conjugated Polymers

Michinobu, Tsuyoshi, Osako, Haruka, Murata, Kimie, Shigehara, Kiyotaka

Chemistry Letters 39 ( 3 ) 2010

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DOI： 10.1246/cl.2010.168

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Synthesis and Properties of 1,8-Carbazole-Based Conjugated Copolymers

Michinobu, Tsuyoshi, Osako, Haruka, Shigehara, Kiyotaka

Polymers 2 ( 3 ) 2010

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DOI： 10.3390/polym2030159

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Synthesis and Characterization of Hybrid Biopolymers of L-lactic Acid and 2-Pyrone-4,6-dicarboxylic Acid

Michinobu, Tsuyoshi, Bito, Masami, Tanimura, Miki, Katayama, Yoshihiro, Masai, Eiji, Nakamura, Masaya, Otsuka, Yuichiro, Ohara, Seiji, Shigehara, Kiyotaka

Journal of Macromolecular Science Part a-Pure and Applied Chemistry 47 ( 6 ) 2010

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DOI： 10.1080/10601321003742121

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Sequential double click reactions: a highly efficient post-functionalization method for optoelectronic polymers

Li, Yongrong, Michinobu, Tsuyoshi

Polymer Chemistry 1 ( 1 ) 2010

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DOI： 10.1039/b9py00238c

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Organogels of Lignin-derived Stable Metabolic Intermediate, 2-Pyrone-4,6-dicarboxylic Acid (PDC), Bearing Cholesteryl Groups

Michinobu, Tsuyoshi, Hiraki, Kenta, Fujii, Nozomu, Shikinaka, Kazuhiro, Katayama, Yoshihiro, Masai, Eiji, Nakamura, Masaya, Otsuka, Yuichiro, Ohara, Seiji, Shigehara, Kiyotaka

Chemistry Letters 39 ( 4 ) 2010

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DOI： 10.1246/cl.2010.400

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The Simplest Layer-by-Layer Assembly Structure: Best Paired Polymer Electrolytes with One Charge per Main Chain Carbon Atom for Multi layered Thin Films

Fujii, Nozomu, Fujimoto, Kouji, Michinobu, Tsuyoshi, Akada, Misaho, Hill, Jonathan P., Shiratori, Seimei, Ariga, Katsuhiko, Shigehara, Kiyotaka

Macromolecules 43 ( 8 ) 2010

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DOI： 10.1021/ma100473j

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Two-dimensionally extended organic high-spin poly(aminium cationic radical)s and their magnetic force microscopic images

Michinobu, Tsuyoshi, Inui, Jun, Nishide, Hiroyuki

Polymer Journal 42 ( 7 ) 2010

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DOI： 10.1038/pj.2010.47

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All-optical high-speed signal processing with silicon-organic hybrid slot waveguidesx Reviewed

C. Koos, P. Vorreau, T. Vallaitis, P. Dumon, W. Bogaerts, R. Baets, B. Esembeson, I. Biaggio, T. Michinobu, F. Diederich, W. Freude, J. Leuthold

NATURE PHOTONICS 3 ( 4 ) 216 - 219 2009.4

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DOI： 10.1038/NPHOTON.2009.25

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Two-Dimensionally Extended Aromatic Polyamines for Optimization of Charge-Transporting Properties by Partial Oxidation

Michinobu, Tsuyoshi, Kato, Fumiaki, Inui, Jun, Nishide, Hiroyuki

Journal of Polymer Science Part a-Polymer Chemistry 47 ( 18 ) 2009

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DOI： 10.1002/pola.23510

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One-Step Synthesis of Donor-Acceptor type Conjugated Polymers from Ferrocene-Containing Poly(aryleneethynylene)s

Michinobu, Tsuyoshi, Kumazawa, Hiroe, Noguchi, Keiichi, Shigehara, Kiyotaka

Macromolecules 42 ( 16 ) 2009

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DOI： 10.1021/ma9013324

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Mechanical Properties of Poly(L-Lactide) Films Controlled by Blending with Polyesters of Lignin-Derived Stable Metabolic Intermediate, 2-Pyrone-4,6-Dicarboxylic Acid (PDC)

Michinobu, Tsuyoshi, Bito, Masami, Tanimura, Miki, Katayama, Yoshihiro, Masai, Eiji, Nakamura, Masaya, Otsuka, Yuichiro, Ohara, Seiji, Shigehara, Kiyotaka

Polymer Journal 41 ( 10 ) 2009

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DOI： 10.1295/polymj.PJ2009133

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Intramolecular Through-Space Antiferromagnetic Interactions of Cross-Conjugated Aromatic Polyaminium Radical Gels

Michinobu, Tsuyoshi, Tanaka, Manabu, Inui, Jun, Nishide, Hiroyuki

Journal of Nanoscience and Nanotechnology 9 ( 1 ) 2009

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DOI： 10.1166/jnn.2009.J020

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Fusible, Elastic, and Biodegradable Polyesters of 2-Pyrone-4,6-Dicarboxylic Acid (PDC)

Michinobu, Tsuyoshi, Bito, Masami, Yamada, Yoshiko, Tanimura, Miki, Katayama, Yoshihiro, Masai, Eiji, Nakamura, Masaya, Otsuka, Yuichiro, Ohara, Seiji, Shigehara, Kiyotaka

Polymer Journal 41 ( 12 ) 2009

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DOI： 10.1295/polymj.PJ2009045R

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All-Optical Wavelength Conversion at 42.7 Gbit/s in a 4 mm Long Silicon-Organic Hybrid Waveguide Reviewed

T. Vallaitis, C. Heine, R. Bonk, W. Freude, J. Leuthold, C. Koos, B. Esembeson, I. Biaggio, T. Michinobu, F. Diederich, P. Dumon, R. Baets

OFC: 2009 CONFERENCE ON OPTICAL FIBER COMMUNICATION, VOLS 1-5 2858 - + 2009

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DOI： 10.1109/PS.2009.5307823

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A High-Optical Quality Supramolecular Assembly for Third-Order Nonlinear Optics Reviewed

Michelle L. Scimeca, Bweh Esembeson, Ivan Biaggio, Tsuyoshi Michinobu, Francois Diederich

2009 CONFERENCE ON LASERS AND ELECTRO-OPTICS AND QUANTUM ELECTRONICS AND LASER SCIENCE CONFERENCE (CLEO/QELS 2009), VOLS 1-5 3005 - + 2009

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Synthesis and Properties of Conjugated Poly(1,8-carbazole)s

Michinobu, Tsuyoshi, Osako, Haruka, Shigehara, Kiyotaka

Macromolecules 42 ( 21 ) 2009

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DOI： 10.1021/ma901502b

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Supramolecular Shape Shifter: Polymorphs of Self-Organized Fullerene Assemblies

Nakanishi, Takashi, Wang, Jiaobing, Moehwald, Helmuth, Kurth, Dirk G., Michinobu, Tsuyoshi, Takeuchi, Masayuki, Ariga, Katsuhiko

Journal of Nanoscience and Nanotechnology 9 ( 1 ) 2009

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DOI： 10.1166/jnn.2009.J030

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Vapor deposited small molecules as an organic nonlinear optical cladding for silicon on insulator technology Reviewed

Ivan Biaggio, Michelle L. Scimeca, Bweh Esembeson, T. Michinobu, F. Diederich, C. Koos, W. Freude, J. Leuthold

2009 CONFERENCE ON LASERS AND ELECTRO-OPTICS AND QUANTUM ELECTRONICS AND LASER SCIENCE CONFERENCE (CLEO/QELS 2009), VOLS 1-5 209 - + 2009

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Synthesis and Properties of Nitrogen-Linked Poly(2,7-carbazole)s as Hole-Transport Material for Organic Light Emitting Diodes

Michinobu, Tsuyoshi, Kumazawa, Hiroe, Otsuki, Eiji, Usui, Hiroaki, Shigehara, Kiyotaka

Journal of Polymer Science Part a-Polymer Chemistry 47 ( 15 ) 2009

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DOI： 10.1002/pola.23454

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Silicon-organic hybrid (SOH) devices for nonlinear optical signal processing Reviewed

W. Freude, J. -M Brosi, C. Koos, P. Vorreau, L. C. Andreani, P. Dumon, R. Baets, B. Esembeson, I. Biaggio, T. Michinobu, F. Diederich, J. Leuthold

ICTON 2008: PROCEEDINGS OF 2008 10TH ANNIVERSARY INTERNATIONAL CONFERENCE ON TRANSPARENT OPTICAL NETWORKS, VOL 2 84 - + 2008

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DOI： 10.1109/ICTON.2008.4598598

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A novel biomass-based polymer prepared from lignin-derived stable metabolic intermediate by copper(I)-catalyzed azide-alkyne click reaction

Michinobu, Tsuyoshi, Inazawa, Yasunori, Hiraki, Kenta, Katayama, Yoshihiro, Masai, Eiji, Nakamura, Masaya, Ohara, Seiji, Shigehara, Kiyotaka

Chemistry Letters 37 ( 2 ) 2008

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DOI： 10.1246/cl.2008.154

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A High-Optical Quality Supramolecular Assembly for Third-Order Integrated Nonlinear Optics

Esembeson, Bweh, Scimeca, Michelle L., Michinobu, Tsuyoshi, Diederich, Francois, Biaggio, Ivan

Advanced Materials 20 ( 23 ) 2008

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DOI： 10.1002/adma.200801552

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One-electron-reduced and -oxidized stages of donor-substituted 1,1,4,4-tetracyanobuta-1,3-dienes of different molecular architectures

Kivala, Milan, Stanoeva, Tsvetanka, Michinobu, Tsuyoshi, Frank, Brian, Gescheidt, Georg, Diederich, Francois

Chemistry-a European Journal 14 ( 25 ) 2008

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DOI： 10.1002/chem.200800716

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Nanocarbon superhydrophobic surfaces created from fullerene-based hierarchical supramolecular assemblies

Nakanishi, Takashi, Michinobu, Tsuyoshi, Yoshida, Kaname, Shirahata, Naoto, Ariga, Katsuhiko, Moehwald, Helmuth, Kurth, Dirk G.

Advanced Materials 20 ( 3 ) 2008

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DOI： 10.1002/adma.200701537

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Band-gap tuning of carbazole-containing donor-acceptor type conjugated polymers by acceptor moieties and pi-spacer groups

Michinobu, Tsuyoshi, Okoshi, Kensuke, Sako, Haruka, Kumazawa, Hiroe, Shigehara, Kiyotaka

Polymer 49 ( 1 ) 2008

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DOI： 10.1016/j.polymer.2007.11.022

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Alkyne-linked poly(1,8-carbazole)s: A novel class of conjugated carbazole polymers

Michinobu, Tsuyoshi, Osako, Haruka, Shigehara, Kiyotaka

Macromolecular Rapid Communications 29 ( 2 ) 2008

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DOI： 10.1002/marc.200700715

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Fine-tuning supramolecular assemblies of fullerenes bearing long alkyl chains

Nakanishi, Takashi, Takahashi, Hirokazu, Michinobu, Tsuyoshi, Hill, Jonathan P., Teranishi, Toshiharu, Ariga, Katsuhiko

Thin Solid Films 516 ( 9 ) 2008

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DOI： 10.1016/j.tsf.2007.04.110

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Click-Type Reaction of Aromatic Polyamines for Improvement of Thermal and Optoelectronic Properties

Michinobu, Tsuyoshi

Journal of the American Chemical Society 130 ( 43 ) 2008

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DOI： 10.1021/ja8061612

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Chiral recognition at the air-water interface

Ariga, Katsuhiko, Michinobu, Tsuyoshi, Nakanishi, Takashi, Hill, Jonathan P.

Current Opinion in Colloid & Interface Science 13 ( 1-2 ) 2008

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DOI： 10.1016/j.cocis.2007.08.010

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Radical polymerization of fumaramide and fumaramate derivatives for homogeneous Langmuir monolayers

Michinobu, Tsuyoshi, Nakada, Kazuya, Shigehara, Kiyotaka

Polymer Bulletin 60 ( 1 ) 2008

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DOI： 10.1007/s00289-007-0839-9

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Polyesters of 2-pyrone-4,6-dicarboxylic acid (PDC) obtained from a metabolic intermediate of lignin

Michinobu, Tsuyoshi, Hishida, Masakiyo, Sato, Masae, Katayama, Yoshihiro, Masai, Eiji, Nakamura, Masaya, Otsuka, Yuichiro, Ohara, Seiji, Shigehara, Kiyotaka

Polymer Journal 40 ( 1 ) 2008

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DOI： 10.1295/polymj.PJ2007158

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Molecular orientation in Langmuir-Blodgett films of polyfumarates carrying isopropylester and isopropylamide side chains

Michinobu, Tsuyoshi, Nakada, Kazuya, Matsuda, Masaki, Shigehara, Kiyotaka

Colloids and Surfaces a-Physicochemical and Engineering Aspects 321 ( 1-3 ) 2008

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DOI： 10.1016/j.colsurfa.2007.12.014

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Fullerene nanowires on graphite: Epitaxial self-organizations of a fullerene bearing double long-aliphatic chains

Nakanishi, Takashi, Takahashi, Hirokazu, Michinobu, Tsuyoshi, Takeuchi, Masayuki, Teranishi, Toshiharu, Ariga, Katsuhiko

Colloids and Surfaces a-Physicochemical and Engineering Aspects 321 ( 1-3 ) 2008

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DOI： 10.1016/j.colsurfa.2007.11.029

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Highly Nonlinear Silicon Photonics Slot Waveguides without Free Carrier Absorption Related Speed-Limitations Reviewed

T. Vallaitis, C. Koos, B. Esembeson, I. Biaggio, T. Michinobu, F. Diederich, P. Dumon, R. Baets, W. Freude, J. Leuthold

2008 34TH EUROPEAN CONFERENCE ON OPTICAL COMMUNICATION (ECOC) 2008

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DOI： 10.1109/ECOC.2008.4729411

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Unexpected phase Behaviors of poly(fumarate)s carrying tolane-based mesogenic side chains

Michinobu, Tsuyoshi, Noguchi, Hiroshi, Fujii, Nozomu, Tokita, Masatoshi, Watanabe, Junji, Shigehara, Kiyotaka

Chemistry Letters 37 ( 3 ) 2008

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Publishing type：Research paper (scientific journal)

DOI： 10.1246/cl.2008.356

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Thermoreversible Contraction and Extension of Layer Spacing in Smectic Phase of Side Chain Liquid Crystal Poly(fumarate)s

Michinobu, Tsuyoshi, Fujii, Nozomu, Tokita, Masatoshi, Watanabe, Junji, Shigehara, Kiyotaka

Macromolecular Rapid Communications 29 ( 19 ) 2008

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DOI： 10.1002/marc.200800363

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Side chain liquid crystal poly(fumarate)s rearing tolane-based mesogens

Noguchi, Hiroshi, Michinobu, Tsuyoshi, Fujii, Nozomu, Funahashi, Masahiro, Tokita, Masatoshi, Watanabe, Junji, Shigehara, Kiyotaka

Journal of Polymer Science Part a-Polymer Chemistry 46 ( 15 ) 2008

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DOI： 10.1002/pola.22838

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Molecular properties of 2-pyrone-4,6-dicarboxylic acid (PDC) as a stable metabolic intermediate of lignin isolated by fractional precipitation with Na+ ion

Michinobu, Tsuyoshi, Bito, Masami, Yamada, Yoshiko, Katayama, Yoshihiro, Noguchi, Keiichi, Masai, Eiji, Nakamura, Masaya, Ohara, Seiji, Shigehara, Kiyotaka

Bulletin of the Chemical Society of Japan 80 ( 12 ) 2007

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DOI： 10.1246/bcsj.80.2436

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Synthesis and the phase behavior of liquid-crystalline fumarates bearing tolane-based mesogens

Noguchi, Hiroshi, Michinobu, Tsuyoshi, Shigehara, Kiyotaka

Chemistry Letters 36 ( 8 ) 2007

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Publishing type：Research paper (scientific journal)

DOI： 10.1246/cl.2007.1044

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Flower-shaped supramolecular assemblies: Hierarchical organization of a fullerene bearing long aliphatic chains

Nakanishi, Takashi, Ariga, Katsuhiko, Michinobu, Tsuyoshi, Yoshida, Kaname, Takahashi, Hirokazu, Teranishi, Toshiharu, Moehwald, Helmuth, Kurth, Dirk G.

Small 3 ( 12 ) 2007

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Publishing type：Research paper (scientific journal)

DOI： 10.1002/smll.200700647

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Control of phase-transition behavior and polymerization capability by methyl addition to dialkyl fumarates bearing cyanobiphenyl mesogens

Fujii, Nozomu, Michinobu, Tsuyoshi, Shigehara, Kiyotaka

Chemistry Letters 36 ( 8 ) 2007

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Publishing type：Research paper (scientific journal)

DOI： 10.1246/cl.2007.1052

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Synthesis,and optical properties of carbazole-containing donor-acceptor type conjugated polymers

Michinobu, Tsuyoshi, Okoshi, Kensuke, Osako, Haruka, Kumazawa, Hiroe, Shigehara, Kiyotaka

Journal of Photopolymer Science and Technology 20 ( 2 ) 2007

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DOI： 10.2494/photopolymer.20.255

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Phase transition behavior in side-chain liquid crystal polymers of different chain-backbones

Fujii, Nozomu, Kawase, Yasunori, Michinobu, Tsuyoshi, Shigehara, Kiyotaka

Journal of Photopolymer Science and Technology 20 ( 1 ) 2007

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Publishing type：Research paper (scientific journal)

DOI： 10.2494/photopolymer.20.17

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Nitrogen-linked aromatic poly(2,7-carbazole)s: Partially annulated poly(m-aniline)s

Michinobu, Tsuyoshi, Kumazawa, Hiroe, Shigehara, Kiyotaka

Chemistry Letters 36 ( 5 ) 2007

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DOI： 10.1246/cl.2007.620

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Immobilization of biomaterials to nano-assembled films (self-assembled monolayers, Langmuir-Blodgett films, and layer-by-layer assemblies) and their related functions

Ariga, Katsuhiko, Nakanishi, Takashi, Michinobu, Tsuyoshi

Journal of Nanoscience and Nanotechnology 6 ( 8 ) 2006

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Publishing type：Research paper (scientific journal)

DOI： 10.1166/jnn.2006.503

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Donor-substituted 1,1,4,4-tetracyanobutadienes (TCBDs): New chromophores with efficient intramolecular charge-transfer interactions by atom-economic synthesis

Michinobu, T, Boudon, C, Gisselbrecht, JP, Seiler, P, Frank, B, Moonen, NNP, Gross, M, Diederich, F

Chemistry-a European Journal 12 ( 7 ) 2006

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Publishing type：Research paper (scientific journal)

DOI： 10.1002/chem.200501113

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Room temperature liquid fullerenes: An uncommon morphology of C-60 derivatives

Michinobu, Tsuyoshi, Nakanishi, Takashi, Hill, Jonathan P., Funahashi, Masahiro, Ariga, Katsuhiko

Journal of the American Chemical Society 128 ( 32 ) 2006

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DOI： 10.1021/ja063866z

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Perfectly straight nanowires of fullerenes bearing long alkyl chains on graphite

Nakanishi, Takashi, Miyashita, Naoko, Michinobu, Tsuyoshi, Wakayama, Yutaka, Tsuruoka, Tohru, Ariga, Katsuhiko, Kurth, Dirk G.

Journal of the American Chemical Society 128 ( 19 ) 2006

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Publishing type：Research paper (scientific journal)

DOI： 10.1021/ja061450f

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Mechanical control of enantioselectivity of amino acid recognition by cholesterol-armed cyclen monolayer at the air-water interface

Michinobu, Tsuyoshi, Shinoda, Satoshi, Nakanishi, Takashi, Hill, Jonathan P., Fujii, Kazuko, Player, Tomoko N., Tsukube, Hiroshi, Ariga, Katsuhiko

Journal of the American Chemical Society 128 ( 45 ) 2006

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Publishing type：Research paper (scientific journal)

DOI： 10.1021/ja066429t

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Crystalline thin film of a donor-substituted cyanoethynylethene for nanoscale data recording through intermolecular charge-transfer interactions

Jiang, GY, Michinobu, T, Yuan, WF, Teng, M, Wen, YQ, Du, SX, Gao, HJ, Jiang, L, Song, YL, Diederich, F, Zhu, DB

Advanced Materials 17 ( 18 ) 2005

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Publishing type：Research paper (scientific journal)

DOI： 10.1002/adma.200500559

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A new class of organic donor-acceptor molecules with large third-order optical nonlinearities

Michinobu, T, May, JC, Lim, JH, Boudon, C, Gisselbrecht, JP, Seiler, P, Gross, M, Biaggio, I, Diederich, F

Chemical Communications ( 6 ) 2005

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Publishing type：Research paper (scientific journal)

DOI： 10.1039/b417393g

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Highly efficient third-order optical nonlinearities in donor-substituted cyanoethynylethene molecules

May, JC, Lim, JH, Biaggio, I, Moonen, NNP, Michinobu, T, Diederich, F

Optics Letters 30 ( 22 ) 2005

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Publishing type：Research paper (scientific journal)

DOI： 10.1364/OL.30.003057

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Hierarchical supramolecular fullerene architectures with controlled dimensionality

Nakanishi, T, Schmitt, W, Michinobu, T, Kurth, DG, Ariga, K

Chemical Communications ( 48 ) 2005

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Publishing type：Research paper (scientific journal)

DOI： 10.1039/b512320h

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Microparticles of poly(methacrylic acid) - Gadolinium ion complex and their magnetic force microscopic images

Michinobu, T, Sasao, N, Nishide, H

Journal of Polymer Science Part a-Polymer Chemistry 42 ( 8 ) 2004

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Publishing type：Research paper (scientific journal)

DOI： 10.1002/pola.20029

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Nanometer-size multispin macromolecules and their magnetic force microscopic images Reviewed

Michinobu T, Nishide H, Ueyama N, Harada A

Macromolecular Nanostructured Materials 78 66 - 79 2004

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Other Link： http://orcid.org/0000-0001-6948-1189
m-phenylene-linked aromatic poly(aminium cationic radical)s: Persistent high-spin organic polyradicals

Michinobu, T, Inui, J, Nishide, H

Organic Letters 5 ( 12 ) 2003

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Publishing type：Research paper (scientific journal)

DOI： 10.1021/ol0346281

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Preparation of non-Kekule- and nondisjoint-type aromatic polyamines by palladium-catalyzed polycondensation and their poly(cationic radical)s

Michinobu, T, Inui, J, Nishide, H

Polyhedron 22 ( 14-17 ) 2003

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Publishing type：Research paper (scientific journal)

DOI： 10.1016/S0277-5387(03)00170-0

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Magnetic force microscopic images of nanometer-sized polyradical particles

Michinobu, T, Inui, J, Nishide, H

Polymer Journal 35 ( 1 ) 2003

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Publishing type：Research paper (scientific journal)

DOI： 10.1295/polymj.35.71

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5,4 '-Bis[bis(methoxyphenyl)amino]-2-methoxystilbene and its cationic biradical

Michinobu, T, Tsuchida, E, Nishide, H

Polyhedron 20 ( 11-14 ) 2001

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Publishing type：Research paper (scientific journal)

DOI： 10.1016/S0277-5387(01)00586-1

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3,4 '-bis[bis(t-butyl- and methoxy-phenyl)amino]stilbene bis(cation radical)s and their electrochemical and magnetic properties

Michinobu, T, Tsuchida, E, Nishide, H

Bulletin of the Chemical Society of Japan 73 ( 4 ) 2000

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Publishing type：Research paper (scientific journal)

DOI： 10.1246/bcsj.73.1021

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Robust triplet molecule: Cationic diradical of 3,4 '-bis(diphenylamino)stilbene

Michinobu, T, Takahashi, M, Tsuchida, E, Nishide, H

Chemistry of Materials 11 ( 8 ) 1999

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DOI： 10.1021/cm990295j

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Books

Routledge Resources Online: Polymers, Polymeric Materials, and Polymer Technology

（ Role： Joint translator , Original_author： T. Michinobu, H. Jia, N. Yomogita , https://doi.org/10.1201/9780367694265-EPPMPT99-1）

CRC Press 2025.3

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Optical and Optoelectronic Polymers

K. Terayama, T. Michinobu（ Role： Joint authorpp. 435-457）

Royal Society of Chemistry 2024.10

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微生物を用いた有用物質生産技術の開発

中村雅哉, 荒木拓馬, 鈴木悠造, 大塚祐一郎, 政井英司, 上村直史, 道信剛志, 敷中一洋, 片山義博（ Role： Joint authorpp. 352-361）

技術情報協会 2024.6 （ ISBN:9784867980231 ）

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Total pages：442p Language：Japanese

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生分解性プラスチックの開発と市場 = Development and market of biodegradable plastics

道信剛志, 金易介, 上村直史, 政井英司, 中村雅哉（ Role： Joint authorpp. 30-36）

シーエムシー出版 2024.5 （ ISBN:9784781317960 ）

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Total pages：v, 190p Language：Japanese

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有機半導体の開発と最新動向

道信剛志（ Role： Joint authorpp. 109-116）

シーエムシー出版 2024.3 （ ISBN:9784781317632 ）

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Total pages：xii, 400p Language：Japanese

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ラジカル重合ハンドブック

道信剛志（ Role： Joint authorpp. 606-615）

エヌ・ティー・エス 2023.12 （ ISBN:9784860438715 ）

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Total pages：29, [4], 3, 14, 946, 21p Language：Japanese

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Ambipolar Materials and Devices

T. Michinobu（ Role： Joint author , Original_author： T. Michinobu , pp. 14-26）

Royal Society of Chemistry 2020.9

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ラジカル重合を中心としたポリマー・微粒子・コーティング材の合成、応用、トラブル対策

道信剛志（ Role： Joint authorpp. 316-325）

技術情報協会 2020.2 （ ISBN:9784861047763 ）

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Total pages：658p Language：Japanese

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Encyclopedia of Polymer Applications

T. Michinobu, Y. Wang（ Role： Joint authorpp. 2291-2305）

Taylor & Francis 2019.1

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Optical Properties of Functional Polymers and Nano Engineering Applications

T. Michinobu, T. Hyakutake（ Role： Joint author , Original_author： T. Michinobu, T. Hyakutake , pp. 87-104）

CRC Press 2017.7

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Polymer-Engineered Nanostructures for Advanced Energy Applications

Y. Wang, T. Michinobu（ Role： Joint authorpp. 607-633）

Springer 2017.6

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Organometallics and Related Molecules for Energy Conversion

T. Michinobu（ Role： Joint authorpp. 115-135）

Springer 2015.4

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クリックケミストリー : 基礎から実用まで

道信剛志（ Role： Joint authorpp. 51-60）

シーエムシー出版 2014.8 （ ISBN:9784781309545 ）

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Total pages：viii, 260p Language：Japanese

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Dynamic Functions at Molecularly-Assembled Films

K. Ariga, T. Nakanishi, T. Michinobu（ Role： Joint authorpp. 109-140）

American Scientific Publishers 2009

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フラーレン超分子の微細加工技術と展望

中西尚志, 道信剛志（ Role： Joint authorpp. 695-699）

エヌ・ティー・エス 2007

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Nanometer-Sized Multi-Spin Macromolecules and their Magnetic Force Microscopic Images

T. Michinobu, H. Nishide（ Role： Joint authorpp. 66-79）

Kodansha 2004

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MISC

画像技術を支える高分子の基礎（Ⅷ）―アルキン含有半導体ポリマーの合成と薄膜電子デバイス応用― Invited

道信剛志, 磯辺篤

日本画像学会誌 64 ( 3 ) 293 - 300 2025.3

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クリックケミストリーを利用した機能性繊維・高分子材料の創製 Invited

道信剛志

繊維学会誌 80 ( 8 ) 243 - 247 2024.8

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クリックケミストリーによる高分子合成技術の開発動向 Invited

道信剛志

塗装工学 58 ( 9 ) 364 - 371 2023.9

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[2+2]付加環化反応を用いた機能性コーティング材料の開発 Invited Reviewed

道信剛志

材料表面 7 ( 4 ) 162 - 168 2022.12

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電子のみを輸送する半導体高分子の合成と応用－全有機高分子から成る次世代電子デバイスの可能性 Invited

道信剛志

化学 75 ( 1 ) 70 - 71 2020.1

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クリックケミストリーによる新高分子材料合成 Invited

道信剛志

機能材料 38 ( 9 ) 12 - 20 2018.9

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クリックケミストリーを用いた高分子合成 Invited Reviewed

道信剛志

化学と教育 65 ( 3 ) 444 - 445 2017.9

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新しい高分子・繊維材料の創製と機能発現のための道筋 Invited Reviewed

道信剛志

繊維学会誌 72 ( 7 ) 333 - 334 2016.7

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Novel Design and Organic Device Applications of n-Type Semiconducting Polymers

115 ( 485 ) 11 - 14 2016.3

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ひび割れを光検出する塗料と構造物劣化検出

百武壮, 西崎到, 道信剛志

土木技術資料 57 ( 12 ) 30 - 33 2015.12

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ひび割れ検出塗料を用いた構造物の劣化検出技術

百武壮, 西崎到, 道信剛志

検査技術 20 ( 1 ) 51 - 60 2015.1

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イオン認識能を有する機能性高分子のクリック合成

道信剛志

有機合成化学協会誌 71 ( 2 ) 149 - 157 2013.2

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TCNE-アルキン付加反応に基づく新規芳香族系高分子の合成と光電子機能の評価 Invited

道信剛志

高分子 61 ( 11 ) 875 - 876 2012.11

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共役高分子とクリックケミストリーが出会う時

道信剛志

化学と工業 63 ( 6 ) 489 2010

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Recent progress of click chemistry in polymer science

48 ( 3 ) 82 - 91 2010

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Click-Type Reaction of Aromatic Polyamines

Tsuyoshi Michinobu

58 ( 7 ) 453 2009

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クリックケミストリーを用いたリグニン分解中間物質からなる高分子の合成

道信剛志, 重原淳孝

未来材料 9 ( 8 ) 36 - 43 2009

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2-Pyranone-4,6-dicarboxylic acid as a source of green-plastics and anti-bacterial chemicals

Masami Bito, Tsuyoshi Michinobu, Yoshihiro Katayama, Yuichiro Otsuka, Masaya Nakamura, Seiji Ohara, Eiji Masai, Kiyotaka Shigehara

Trans. Mater. Res. Soc. Jpn. 33 ( 4 ) 1165 - 1168 2008

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2-Pyranone-4,6-dicarboxylic acid as a source of green-plastics and anti-bacterial chemicals

Masami Bito, Tsuyoshi Michinobu, Yoshihiro Katayama, Yuichiro Otsuka, Masaya Nakamura, Seiji Ohara, Eiji Masai, Kiyotaka Shigehara

Trans. Mater. Res. Soc. Jpn. 33 ( 4 ) 1165 - 1168 2008

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二次電池特にリチウムイオンバッテリーを中心として

大越健介, 道信剛志, 重原淳孝

化学と教育 56 ( 3 ) 2 - 6 2008

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液晶性ポリフマレート

道信剛志, 藤井望, 重原淳孝

表面 46 ( 4 ) 169 - 177 2008

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Phase Transition Behaviors in Liquid Crystalline Poly(fumarate)s of Different Mesogen Density

Nozomu Fujii, Yasunori Kawase, Tsuyoshi Michinobu, Kiyotaka Shigehara

TRANSACTIONS OF THE MATERIALS RESEARCH SOCIETY OF JAPAN, VOL 33, NO 2 33 ( 2 ) 391 - 394 2008

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Phase Transition Behaviors in Liquid Crystalline Poly(fumarate)s of Different Mesogen Density

Nozomu Fujii, Yasunori Kawase, Tsuyoshi Michinobu, Kiyotaka Shigehara

TRANSACTIONS OF THE MATERIALS RESEARCH SOCIETY OF JAPAN, VOL 33, NO 2 33 ( 2 ) 391 - 394 2008

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縮合多環共役電子系の新しい花形

道信剛志

化学 62 ( 5 ) 57 - 58 2007

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Recent progress of biomass-based polymers

45 ( 7 ) 239 - 246 2007

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Optimizing specific third-order polarizabilities and approaching the fundamental limit in donor substituted cyanoethynylethene (CEE) molecules

Joshua C. May, Philip R. LaPorta, Bweh Esembeson, Ivan Biaggio, Tsuyoshi Michinobu, Filip Bures, Francois Diederich

LINEAR AND NONLINEAR OPTICS OF ORGANIC MATERIALS VI 6331 633101/1-633101/14 2006

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DOI： 10.1117/12.683451

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Optimizing specific third-order polarizabilities and approaching the fundamental limit in donor substituted cyanoethynylethene (CEE) molecules

Joshua C. May, Philip R. LaPorta, Bweh Esembeson, Ivan Biaggio, Tsuyoshi Michinobu, Filip Bures, Francois Diederich

LINEAR AND NONLINEAR OPTICS OF ORGANIC MATERIALS VI 6331 633101/1-633101/14 - 33101 2006

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DOI： 10.1117/12.683451

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Presentations

Polyurethane Adhesives Based on Lignin-Derived 2-Pyrone-4,6-Dicarboxylic Acid

Y. Cheng, T. Araki, N. Kamimura, E. Masai, M. Nakamura, S. Manzhos, T. Michinobu

International Symposium on Fiber Science and Technology 2024 (ISF2024) 2024.11

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Event date： 2024.11

Language：English Presentation type：Poster presentation

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Biodegradable and Adhesive Properties of Biomass-Based Polymers Containing 2-Pyrone-4,6-Dicarboxylic Acid

Y. Jin, T. Araki, N. Kamimura, E. Masai, M. Nakamura, T. Michinobu

International Symposium on Fiber Science and Technology 2024 (ISF2024) 2024.11

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Event date： 2024.11

Language：English Presentation type：Oral presentation (general)

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Heat-Resistant Silicone Rubber with Lignin-Derived 2-Pyrone-4,6-Dicarboxylic Acid as a Chain Extender and Crosslinker

T. Shimura, T. Araki, N. Kamimura, E. Masai, M. Nakamura, T. Michinobu

International Symposium on Fiber Science and Technology 2024 (ISF2024) 2024.11

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Event date： 2024.11

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リグニン由来2-ピロン-4，6-ジカルボン酸を含むバイオベースポリマーの合成と生分解性

道信剛志, 金易介, 上村直史, 政井英司, 荒木拓馬, 中村雅哉

第73回高分子討論会 2024.9

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Event date： 2024.9

Language：Japanese Presentation type：Oral presentation (general)

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Synthesis of Water-soluble Cyano-containing Polymeric Additives and Their Application to the Preparation of Ag+-loaded Hydrogels

X. Chen, T. Michinobu

第73回高分子討論会 2024.9

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Event date： 2024.9

Language：English Presentation type：Oral presentation (general)

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Crosslinked Donor-Acceptor Electrets and Solution-Processed Polymer Transistor Memories Invited

T. Michinobu, W. He

The International Conference on Flexible and Printed Electronics (ICFPE 2024) 2024.8

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Event date： 2024.8

Language：English Presentation type：Oral presentation (invited, special)

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Biodegradability and Wood Adhesive Properties of Lignin-Derived 2-Pyrone-4,6-Dicarboxylic Acid (PDC) Polyesters

Y. Jin, T. Araki, N. Kamimura, E. Masai, M. Nakamura, T. Michinobu

Polymer Engineering & Science International (PESI) Conference 2024 2024.7

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Event date： 2024.7

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Silicone Rubber with Lignin-Derived 2-Pyrone-4,6-Dicarboxylic Acid

T. Shimura, Y. Jin, T. Araki, N. Kamimura, E. Masai, M. Nakamura, T. Michinobu

Polymer Engineering & Science International (PESI) Conference 2024 2024.7

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Event date： 2024.7

Language：English Presentation type：Poster presentation

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2-ピロン-4,6-ジカルボン酸を含むバイオマス高分子の合成と接着特性

道信剛志, 金易介, 上村直史, 政井英司, 荒木拓馬, 中村雅哉

2024年繊維学会年次大会 2024.6

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Event date： 2024.6

Language：Japanese Presentation type：Oral presentation (general)

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クリックケミストリーを利用した機能性繊維・高分子材料の創製 Invited

道信剛志

2024年繊維学会年次大会 2024.6

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Event date： 2024.6

Language：Japanese Presentation type：Oral presentation (invited, special)

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Solution-Processed Polymer Transistor Memories Invited

T. Michinobu, W. He

IUMRS-ICEM2024 2024.5

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Event date： 2024.5

Language：English Presentation type：Oral presentation (invited, special)

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リグニン由来2-ピロン-4,6-ジカルボン酸（PDC）から成る木材接着剤ポリエステルの開発と生分解性評価

金易介, 荒木拓馬, 上村直史, 政井英司, 中村雅哉, 道信剛志

日本化学会第104春季年会(2024) 2024.3

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Event date： 2024.3

Language：Japanese Presentation type：Poster presentation

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Push-Pull Chromophores with Different Heterocyclic Donor Moieties Synthesized by [2+2] Cycloaddition-Retroelectrocyclization Reaction

X. Chen, T. Michinobu

日本化学会第104春季年会(2024) 2024.3

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Event date： 2024.3

Language：English Presentation type：Poster presentation

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Solar-Driven Steam Generation Properties of Donor-Acceptor Molecules Functionalized by [2+2] Cycloaddition-Retroelectrocyclization Reactions

C.-Y. Lin, T. Michinobu

日本化学会第104春季年会(2024) 2024.3

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Event date： 2024.3

Language：English Presentation type：Poster presentation

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Industrial property rights

機能性ネットワークポリマー組成物

道信剛志, 藤田弘幸, 仁平南帆子

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Applicant：株式会社J−ケミカル

Application no：特願2012-121886 Date applied：2012.5

Announcement no：特開2013-245330 Date announced：2013.12

Patent/Registration no：特許第5798979号 Date issued：2015.8

J-GLOBAL

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機能性ネットワークポリマー組成物

道信剛志, 藤田弘幸, 仁平南帆子

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Applicant：株式会社J−ケミカル

Application no：特願2012-121886 Date applied：2012.5

Announcement no：特開2013-245330 Date announced：2013.12

J-GLOBAL

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化合物合成方法、高分子化合物および環状化合物

道信剛志, 鷲野佑輔

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Applicant：国立大学法人東京工業大学

Application no：特願2012-554704 Date applied：2012.1

Patent/Registration no：特許第5411995号 Date issued：2013.11

J-GLOBAL

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化合物合成方法、高分子化合物および環状化合物

道信剛志, 鷲野佑輔

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Applicant：国立大学法人東京工業大学

Application no：JP2012000554 Date applied：2012.1

Announcement no：WO2012-102061 Date announced：2012.8

J-GLOBAL

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高分子化合物及び電子素子

道信剛志, 原宇平, 加藤岳仁, 三宅邦仁

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Applicant：住友化学株式会社, 国立大学法人東京工業大学

Application no：特願2011-268114 Date applied：2011.12

Announcement no：特開2013-119589 Date announced：2013.6

J-GLOBAL

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高分子化合物の製造方法

道信剛志, 原宇平, 三宅邦仁

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Applicant：国立大学法人東京工業大学, 住友化学株式会社

Application no：特願2011-133452 Date applied：2011.6

Announcement no：特開2012-021150 Date announced：2012.2

J-GLOBAL

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高分子膜及びガスバリア材

百武壮, 道信剛志, 李永榮

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Applicant：独立行政法人土木研究所

Application no：特願2010-242549 Date applied：2010.10

Announcement no：特開2012-092269 Date announced：2012.5

J-GLOBAL

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高分子膜及びガスバリア材

百武壮, 道信剛志, 李永榮

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Applicant：国立研究開発法人土木研究所

Application no：特願2010-242549 Date applied：2010.10

Announcement no：特開2012-092269 Date announced：2012.5

Patent/Registration no：特許第5733816号 Date issued：2015.4

J-GLOBAL

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有機エレクトロルミネッセンス素子および発光装置

道信剛志, 上谷保則

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Applicant：国立大学法人東京工業大学, 住友化学株式会社

Application no：特願2010-238588 Date applied：2010.10

Announcement no：特開2012-094583 Date announced：2012.5

J-GLOBAL

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高分子化合物及びそれを用いた光電変換素子

道信剛志, 原宇平, 三宅邦仁, 加藤岳仁

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Applicant：国立大学法人東京工業大学, 住友化学株式会社

Application no：特願2010-120819 Date applied：2010.5

Announcement no：特開2011-246594 Date announced：2011.12

J-GLOBAL

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縮環芳香族高分子およびその製造方法

道信剛志, 王冬

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Applicant：国立大学法人東京工業大学

Application no：特願2010-017443 Date applied：2010.1

Announcement no：特開2011-153117 Date announced：2011.8

J-GLOBAL

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フラーレン高分子およびその製造方法

道信剛志

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Applicant：国立大学法人東京工業大学, 国立大学法人東京農工大学

Application no：特願2009-286611 Date applied：2009.12

Announcement no：特開2011-126993 Date announced：2011.6

J-GLOBAL

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光電子機能部位を有する高分子化合物およびその製造方法

道信剛志, リヨンロン

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Applicant：国立大学法人東京工業大学

Application no：特願2009-250942 Date applied：2009.10

Announcement no：特開2011-094066 Date announced：2011.5

J-GLOBAL

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電子状態の制御された共役高分子化合物及びそれを用いた有機半導体材料

道信剛志

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Applicant：国立大学法人東京農工大学

Application no：特願2008-121632 Date applied：2008.5

Announcement no：特開2009-270011 Date announced：2009.11

J-GLOBAL

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液状フラーレン誘導体、その製造方法およびそれを用いた素子

中西尚志, 道信剛志, ヒル, ジョナサンピー, 有賀克彦

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Applicant：独立行政法人物質・材料研究機構

Application no：特願2008-523737 Date applied：2007.7

Patent/Registration no：特許第5121710号 Date issued：2012.11

J-GLOBAL

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液状フラーレン誘導体、その製造方法およびそれを用いた素子

中西尚志, 道信剛志, ヒル, ジョナサンピー, 有賀克彦

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Applicant：独立行政法人物質・材料研究機構

Application no：JP2007063502 Date applied：2007.7

Announcement no：WO2008-004635 Date announced：2008.1

J-GLOBAL

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フラーレン誘導体、フラーレン誘導体の製造方法、ナノ・メゾスコピック材料、および、ナノ・メゾスコピック材料の製造方法

中西尚志, 有賀克彦, 道信剛志, クルス, ディルクジー

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Applicant：独立行政法人物質・材料研究機構

Application no：特願2005-332390 Date applied：2005.11

Announcement no：特開2007-137809 Date announced：2007.6

J-GLOBAL

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二次電池、単量体および重合体

西出宏之, 道信剛志, 岩佐繁之

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Applicant：日本電気株式会社

Application no：特願2003-014816 Date applied：2003.1

Announcement no：特開2004-227946 Date announced：2004.8

J-GLOBAL

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二次電池、単量体および重合体

西出宏之, 道信剛志, 岩佐繁之

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Applicant：日本電気株式会社

Application no：特願2003-014816 Date applied：2003.1

Announcement no：特開2004-227946 Date announced：2004.8

Patent/Registration no：特許第4041973号 Date issued：2007.11

J-GLOBAL

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ラジカル高分子化合物からなる磁性素子

西出宏之, 宮坂誠, 道信剛志

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Applicant：学校法人早稲田大学

Application no：特願2000-279652 Date applied：2000.9

Announcement no：特開2002-093609 Date announced：2002.3

J-GLOBAL

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Awards

繊維学会賞

2024.6 繊維学会クリックケミストリーを利用した機能性繊維・高分子材料の創製

道信剛志

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高分子学会昭和電工マテリアルズ賞

2021.9 高分子学会半導体高分子の電荷輸送および近赤外発光に関する研究

道信剛志

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火薬学会奨励賞

2017.5 火薬学会クリック反応を利用した新しい高窒素含有エネルギーポリマーの合成研究

道信剛志

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有機半導体材料の電子状態変調法に関する研究

2010.6 安藤博記念学術奨励賞有機半導体材料の電子状態変調法に関する研究

道信剛志

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若い世代の特別講演会

2010.3 日本化学会クリック型反応によるドナーアクセプター型共役高分子の合成

道信剛志

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高分子研究奨励賞

2009.5 高分子学会芳香族アミン骨格を用いた機能性高分子の創製

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Research Projects

リグニンから新たな窒素置換化合物を生産するプロセス開発と機能性材料への応用

Grant number：25K02148 2025.4 - 2028.3

日本学術振興会科学研究費助成事業基盤研究(B)

鈴木悠造, 上村直史, 道信剛志

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Grant amount：\25870000 （ Direct Cost: \19900000 、 Indirect Cost：\5970000 ）

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Asymmetric Synthesis of Chiral Nonplanar Polycyclic Aromatic Molecules and Application to Materials Chemistry

Grant number：24H00005 2024.4 - 2031.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for Specially Promoted Research

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Grant amount：\623480000 （ Direct Cost: \479600000 、 Indirect Cost：\143880000 ）

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High-Performance Organic Field-Effect Transistor Memories for Artificial Synapses and Photodetectors

Grant number：23KF0223 2023.11 - 2026.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for JSPS Fellows

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Grant amount：\2100000 （ Direct Cost: \2100000 ）

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Development of BN-embedded naphthalenediimides for high-performance n-type semiconducting polymers

Grant number：23KF0221 2023.11 - 2026.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for JSPS Fellows

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Grant amount：\2100000 （ Direct Cost: \2100000 ）

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Development of Electron-Deficient Organic Semiconductor Polymers Exhibiting the World's Highest Electron Mobility

Grant number：19H02786 2019.4 - 2023.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Grant-in-Aid for Scientific Research (B) Grant-in-Aid for Scientific Research (B)

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Grant amount：\17160000 （ Direct Cost: \13200000 、 Indirect Cost：\3960000 ）

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Organic thin film devices based on narrow bandgap semiconducting polymers

Grant number：18KK0157 2019.2 - 2021.3

Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research Fund for the Promotion of Joint International Research (Fostering Joint International Research (B))

Michinobu Tsuyoshi

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Grant amount：\17680000 （ Direct Cost: \13600000 、 Indirect Cost：\4080000 ）

We have developed new organic semiconductor polymers that can selectively transport electrons. By using an environmentally friendly synthetic method, electron-deficient monomers could be efficiently polymerized. The main chain and side chain structures of the polymers were optimized, resulting in high electron mobilities in the thin film states. It was also found that large-area uniform thin films can be produced at low cost by using the blade-coating method. In addition, the obtained organic semiconductor polymers were applied to organic transistors and all-polymer solar cells, and high electron mobilities and excellent photo-conversion efficiencies were achieved.

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金属触媒を使用しないクリック反応の開発と高分子材料への応用

2015.4 - 2019.3

JSPS 科研費基盤研究(B)

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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[2+2]付加環化における遷移状態の解析と新しいクリック反応の確立

2015.4 - 2018.3

JSPS 科研費基盤研究(C)

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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直接的アリール化重縮合による共役高分子の合成とアニオン認識

2014.4 - 2015.3

JSPS 科研費挑戦的萌芽研究

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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多重クリック反応によるマルチカラー高分子アーキテクチャー

2010.4 - 2014.3

JSPS 科研費若手研究(A)

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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溶媒可溶なフラーレン高分子微粒子の合成とn型半導体特性

2010.4 - 2013.3

JSPS 科研費挑戦的萌芽研究

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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電子注入型水溶性ポリチオフェン誘導体の開発

2009.4 - 2010.3

JST シーズ発掘試験 A:発掘型

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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クリック型反応による有機光電子機能材料の創製

2008.10 - 2012.3

JST さきがけ

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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ドナーアクセプター型共役高分子の「クリック」合成と機能開拓

2008.4 - 2010.3

JSPS 科研費若手研究(B)

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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植物由来原料から創る有機ラジカルポリマーとその二次電池応用

2008.4 - 2009.3

JST シーズ発掘試験 A:発掘型

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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Fine tuning of conjugated systems for organic electronic applications

2008

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Grant type：Competitive

Electronic states and morphology of conjugated systems play an important role in determining the performance of organic electronic devices. In this research program, a new method to tune the electronic states of conjugated molecules is developed.

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圧力・温度・応答ポルフィリンナノワイヤの気水界面での認分子認識

2006.4 - 2008.3

JSPS 科研費若手研究(B)

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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共役アミニウムラジカル高分子の精密合成と室温強磁性

2000.4 - 2003.3

JSPS 特別研究員奨励費

道信剛志

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Authorship：Principal investigator Grant type：Competitive

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